Representability for Quantum Theory beyond Particle-Number Conservation

Fuente: arXiv
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Main Author: Mazziotti, David A.
Format: Preprint
Published: 2026
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author Mazziotti, David A.
author_facet Mazziotti, David A.
contents Representability determines when a two-particle reduced density matrix (2-RDM) corresponds to a physical quantum state, enabling many-particle quantum calculations with 2-RDMs rather than the wave function. In this Letter, we present a solution of the representability problem for quantum systems without particle-number conservation. The physically allowed set of 2-RDMs can be characterized from a geometrically `orthogonal' set, the polar cone. We derive explicit linear equations for the two-body operators in the polar cone -- the intersection of the $p$-positive cone with the two-body operator space -- to obtain a systematic hierarchy of representability conditions that do not depend on higher RDMs or the wave function. Moreover, by augmenting these conditions with the particle-number variance, we obtain a unified framework for treating both particle-number-conserving and nonconserving systems. We illustrate with a spin system and molecular H$_4$.
format Preprint
id arxiv_https___arxiv_org_abs_2604_23869
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Representability for Quantum Theory beyond Particle-Number Conservation
Mazziotti, David A.
Quantum Physics
Chemical Physics
Representability determines when a two-particle reduced density matrix (2-RDM) corresponds to a physical quantum state, enabling many-particle quantum calculations with 2-RDMs rather than the wave function. In this Letter, we present a solution of the representability problem for quantum systems without particle-number conservation. The physically allowed set of 2-RDMs can be characterized from a geometrically `orthogonal' set, the polar cone. We derive explicit linear equations for the two-body operators in the polar cone -- the intersection of the $p$-positive cone with the two-body operator space -- to obtain a systematic hierarchy of representability conditions that do not depend on higher RDMs or the wave function. Moreover, by augmenting these conditions with the particle-number variance, we obtain a unified framework for treating both particle-number-conserving and nonconserving systems. We illustrate with a spin system and molecular H$_4$.
title Representability for Quantum Theory beyond Particle-Number Conservation
topic Quantum Physics
Chemical Physics
url https://arxiv.org/abs/2604.23869