Nuclear non-resonant photoexcitation assisted by electron recombination

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Hauptverfasser: Xue, Nan, Liu, Zuoye, Li, Ziwen, Pálffy, Adriana, Yuan, Jianmin, Wu, Yuanbin, Kong, Xiangjin, Ma, Yu-Gang
Format: Preprint
Veröffentlicht: 2026
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author Xue, Nan
Liu, Zuoye
Li, Ziwen
Pálffy, Adriana
Yuan, Jianmin
Wu, Yuanbin
Kong, Xiangjin
Ma, Yu-Gang
author_facet Xue, Nan
Liu, Zuoye
Li, Ziwen
Pálffy, Adriana
Yuan, Jianmin
Wu, Yuanbin
Kong, Xiangjin
Ma, Yu-Gang
contents We investigate theoretically a nuclear excitation mechanism involving absorption of non-resonant photons leveraged by the coupling to the atomic shell. The nuclear non-resonant photoexcitation is assisted by electron recombination which compensates the energy mismatch between photon and nuclear transition energies, reminiscent of parametric up-conversion in non-linear media. This third-order process proceeds via a virtual nuclear state rather than virtual electronic states, distinguishing this mechanism from the electronic bridge. We investigate the process on the example of a so-far not observed 14.2 keV hard x-ray transition in 193Pt driven by an x-ray free-electron laser. Although the calculated cross section is small, it can be compensated by the vast number of non-resonant photons from the x-ray laser pulse. By enabling nuclear excitation through non-resonant photons, this up-conversion-like mechanism suggests new directions for non-linear x-ray interactions mediated by nuclear transitions.
format Preprint
id arxiv_https___arxiv_org_abs_2604_24045
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Nuclear non-resonant photoexcitation assisted by electron recombination
Xue, Nan
Liu, Zuoye
Li, Ziwen
Pálffy, Adriana
Yuan, Jianmin
Wu, Yuanbin
Kong, Xiangjin
Ma, Yu-Gang
Nuclear Theory
We investigate theoretically a nuclear excitation mechanism involving absorption of non-resonant photons leveraged by the coupling to the atomic shell. The nuclear non-resonant photoexcitation is assisted by electron recombination which compensates the energy mismatch between photon and nuclear transition energies, reminiscent of parametric up-conversion in non-linear media. This third-order process proceeds via a virtual nuclear state rather than virtual electronic states, distinguishing this mechanism from the electronic bridge. We investigate the process on the example of a so-far not observed 14.2 keV hard x-ray transition in 193Pt driven by an x-ray free-electron laser. Although the calculated cross section is small, it can be compensated by the vast number of non-resonant photons from the x-ray laser pulse. By enabling nuclear excitation through non-resonant photons, this up-conversion-like mechanism suggests new directions for non-linear x-ray interactions mediated by nuclear transitions.
title Nuclear non-resonant photoexcitation assisted by electron recombination
topic Nuclear Theory
url https://arxiv.org/abs/2604.24045