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Bibliographic Details
Main Authors: Okuma, Ryutaro, Fujisawa, Yuita, Maekawa, Natsumi, Nakao, Akiko, Ishikawa, Yoshihisa, Kobayashi, Riki, Okada, Yoshinori, Ueta, Daichi
Format: Preprint
Published: 2026
Subjects:
Online Access:https://arxiv.org/abs/2604.25436
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Table of Contents:
  • CeTe$_3$ is a van der Waals antiferromagnet composed of magnetic [CeTe]$^+$ layers coupled to highly conducting Te$^{0.5-}$ square nets. Its simple quasi-two-dimensional electronic structure and cleavable nature make it an appealing platform for exploring correlated magnetism in reduced dimensions. To clarify the nature of its low-temperature state, we performed single-crystal neutron diffraction down to 0.3 K, complemented by scanning tunneling microscopy. A magnetic transition near 1.5 K gives rise to incommensurate Bragg peaks at $q_{\pm}\sim(\pm0.17,0,0.31)$, consistent with a double-$q$ magnetic order whose moments are predominantly aligned along the $c$ axis. The strongly reduced ordered moment is consistent with enhanced quantum fluctuations driven by $c$-$f$ hybridization, while the deviation of the propagation vectors from simple nesting suggests a coupling to residual charge-density-wave instabilities of the quasi-one-dimensional Te-derived bands. These results indicate that CeTe$_3$ hosts a correlated magnetic ground state where spin and itinerant charge degrees of freedom are intimately linked in the van der Waals limit.