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Main Authors: Wang, Yuejian, Wu, Zhongyan, Bhupendra, K C, Zhang, Dongzhou, Wang, Lin, Khare, Sanjay V., Prodan, Lilian, Tsurkan, Vladimir
Format: Preprint
Published: 2026
Subjects:
Online Access:https://arxiv.org/abs/2604.26203
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author Wang, Yuejian
Wu, Zhongyan
Bhupendra, K C
Zhang, Dongzhou
Wang, Lin
Khare, Sanjay V.
Prodan, Lilian
Tsurkan, Vladimir
author_facet Wang, Yuejian
Wu, Zhongyan
Bhupendra, K C
Zhang, Dongzhou
Wang, Lin
Khare, Sanjay V.
Prodan, Lilian
Tsurkan, Vladimir
contents Understanding how electronic transport evolves from localized to itinerant regimes in correlated cluster solids remains an important challenge in condensed-matter physics. Here we investigate the pressure-dependent transport properties of the lacunar spinel GaNb4Se8, a cluster Mott insulator at ambient conditions. At low pressures, the resistivity follows Efros-Shklovskii variable-range hopping, indicating Coulomb-gap-controlled carrier localization (x ~ 6.1 Angstrom). A crossover toward metallic transport begins near ~ 5 GPa, whereas a crystallographic transition from the cubic phase to a monoclinic C2 phase occurs at significantly higher pressure (~ 20 GPa), establishing a hierarchy characterized by the decoupling of electronic delocalization from structural symmetry change. At higher pressures, superconductivity (xi(0) ~ 80-90 Angstrom) emerges from the correlated metallic regime. These results identify GaNb4Se8 as a platform for studying correlation-controlled transport evolution in cluster-based solids.
format Preprint
id arxiv_https___arxiv_org_abs_2604_26203
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle From Wavefunction Collapse to Superconductivity: Evolution of the Electronic State in Compressed GaNb4Se8
Wang, Yuejian
Wu, Zhongyan
Bhupendra, K C
Zhang, Dongzhou
Wang, Lin
Khare, Sanjay V.
Prodan, Lilian
Tsurkan, Vladimir
Superconductivity
Understanding how electronic transport evolves from localized to itinerant regimes in correlated cluster solids remains an important challenge in condensed-matter physics. Here we investigate the pressure-dependent transport properties of the lacunar spinel GaNb4Se8, a cluster Mott insulator at ambient conditions. At low pressures, the resistivity follows Efros-Shklovskii variable-range hopping, indicating Coulomb-gap-controlled carrier localization (x ~ 6.1 Angstrom). A crossover toward metallic transport begins near ~ 5 GPa, whereas a crystallographic transition from the cubic phase to a monoclinic C2 phase occurs at significantly higher pressure (~ 20 GPa), establishing a hierarchy characterized by the decoupling of electronic delocalization from structural symmetry change. At higher pressures, superconductivity (xi(0) ~ 80-90 Angstrom) emerges from the correlated metallic regime. These results identify GaNb4Se8 as a platform for studying correlation-controlled transport evolution in cluster-based solids.
title From Wavefunction Collapse to Superconductivity: Evolution of the Electronic State in Compressed GaNb4Se8
topic Superconductivity
url https://arxiv.org/abs/2604.26203