Universal Nano-Bead Emitter Inks for Programmable Nanometric Fluorescent Architectures

Fuente: arXiv
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Main Authors: Olevsko, Ilya, Shehadeh, Maria, Ohorodniichuk, Dmytro, Weisman, Leonid, Golan, Rotem, Oheim, Martin, Byk, Gerardo, Salomon, Adi
Format: Preprint
Published: 2026
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author Olevsko, Ilya
Shehadeh, Maria
Ohorodniichuk, Dmytro
Weisman, Leonid
Golan, Rotem
Oheim, Martin
Byk, Gerardo
Salomon, Adi
author_facet Olevsko, Ilya
Shehadeh, Maria
Ohorodniichuk, Dmytro
Weisman, Leonid
Golan, Rotem
Oheim, Martin
Byk, Gerardo
Salomon, Adi
contents Fabricating brightly fluorescent layers with nanometric thickness and digitally controlled lateral structuration remains a challenge for next-generation photonic devices, optical calibration standards, and biocompatible interfaces. Here, we introduce Nano-Bead Emitters (NBEs), hydrogel nanoparticles covalently functionalized with fluorophores, as a universal, water-processable ink platform for fabricating programmable nanometric fluorescent architectures. By immobilizing fluorophores within a charged nanohydrogel scaffold, the platform entirely decouples film morphology from dye solubility. This molecule-independent strategy enables spectrally distinct, inherently water-insoluble dyes to be processed using a single, standardized aqueous ink formulation. Combined with laser-induced forward transfer (LIFT) printing, this additive approach yields highly uniform fluorescent layers (~7 nm thickness, sub-nanometric roughness). This structural invariance produces complex multicolor patterns sharing identical thickness and surface morphology across all spectral channels, a critical requirement for quantitative optical calibration. Furthermore, LIFT printing provides programmable, layer-by-layer control over fluorescence intensity via successive deposition cycles, yielding precisely tunable brightness without aggregation-caused quenching. This maskless technique enables rapid, high-fidelity printing of both monochromatic and multicolor patterns over macroscopic areas with absolute spatial resolution. Finally, these universally compatible NBE inks stably deposit onto diverse substrates (glass, polymers, semiconductors, metasurfaces), effectively bridging scalable manufacturing with high-performance integrated photonic systems.
format Preprint
id arxiv_https___arxiv_org_abs_2604_27726
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Universal Nano-Bead Emitter Inks for Programmable Nanometric Fluorescent Architectures
Olevsko, Ilya
Shehadeh, Maria
Ohorodniichuk, Dmytro
Weisman, Leonid
Golan, Rotem
Oheim, Martin
Byk, Gerardo
Salomon, Adi
Optics
Quantitative Methods
Fabricating brightly fluorescent layers with nanometric thickness and digitally controlled lateral structuration remains a challenge for next-generation photonic devices, optical calibration standards, and biocompatible interfaces. Here, we introduce Nano-Bead Emitters (NBEs), hydrogel nanoparticles covalently functionalized with fluorophores, as a universal, water-processable ink platform for fabricating programmable nanometric fluorescent architectures. By immobilizing fluorophores within a charged nanohydrogel scaffold, the platform entirely decouples film morphology from dye solubility. This molecule-independent strategy enables spectrally distinct, inherently water-insoluble dyes to be processed using a single, standardized aqueous ink formulation. Combined with laser-induced forward transfer (LIFT) printing, this additive approach yields highly uniform fluorescent layers (~7 nm thickness, sub-nanometric roughness). This structural invariance produces complex multicolor patterns sharing identical thickness and surface morphology across all spectral channels, a critical requirement for quantitative optical calibration. Furthermore, LIFT printing provides programmable, layer-by-layer control over fluorescence intensity via successive deposition cycles, yielding precisely tunable brightness without aggregation-caused quenching. This maskless technique enables rapid, high-fidelity printing of both monochromatic and multicolor patterns over macroscopic areas with absolute spatial resolution. Finally, these universally compatible NBE inks stably deposit onto diverse substrates (glass, polymers, semiconductors, metasurfaces), effectively bridging scalable manufacturing with high-performance integrated photonic systems.
title Universal Nano-Bead Emitter Inks for Programmable Nanometric Fluorescent Architectures
topic Optics
Quantitative Methods
url https://arxiv.org/abs/2604.27726