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Main Authors: Du, Tao-Yuan, Li, Hui-Ru, Li, Bo, Lu, Ruifeng
Format: Preprint
Published: 2026
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Online Access:https://arxiv.org/abs/2605.01388
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author Du, Tao-Yuan
Li, Hui-Ru
Li, Bo
Lu, Ruifeng
author_facet Du, Tao-Yuan
Li, Hui-Ru
Li, Bo
Lu, Ruifeng
contents High-harmonic generation (HHG) in strongly correlated Mott insulators is investigated using exact diagonalization and time-dependent density-matrix propagation of a laser-driven one-dimensional Hubbard chain. By projecting onto equilibrium Hubbard bands, we use the doublon population and its dynamics as a diagnostic to analyze intraband (spin-wave-like) and interband (doublon-holon creation) excitation channels. A filling-dependent crossover emerges: Bloch-like intraband response at dilute filling, mixed dynamics at intermediate filling, and interband-dominated HHG with plateau and cutoff near half filling. In the considered parameter range, increasing interaction strength $U$ strongly suppresses interband contributions through the enlarged Mott gap and correlation-induced localization. Intra- and interband current decomposition reveals opposing flows below the Mott gap (Δ_{\mathrm{Mott}}) and selective dephasing suppression of interband coherence, enhancing net doublon accumulation. Time-frequency analysis uncovers the filling-dependent features of quantum trajectories, manifesting in distinct below-Δ_{\mathrm{Mott}} emission. This doublon-based analysis provides a transparent link between equilibrium spin-charge separation and nonequilibrium strong-field response, and clarifies how dephasing modifies interband coherence and doublon accumulation.
format Preprint
id arxiv_https___arxiv_org_abs_2605_01388
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Tracking doublon-holon dynamics in high-harmonic generation from Mott insulators
Du, Tao-Yuan
Li, Hui-Ru
Li, Bo
Lu, Ruifeng
Optics
High-harmonic generation (HHG) in strongly correlated Mott insulators is investigated using exact diagonalization and time-dependent density-matrix propagation of a laser-driven one-dimensional Hubbard chain. By projecting onto equilibrium Hubbard bands, we use the doublon population and its dynamics as a diagnostic to analyze intraband (spin-wave-like) and interband (doublon-holon creation) excitation channels. A filling-dependent crossover emerges: Bloch-like intraband response at dilute filling, mixed dynamics at intermediate filling, and interband-dominated HHG with plateau and cutoff near half filling. In the considered parameter range, increasing interaction strength $U$ strongly suppresses interband contributions through the enlarged Mott gap and correlation-induced localization. Intra- and interband current decomposition reveals opposing flows below the Mott gap (Δ_{\mathrm{Mott}}) and selective dephasing suppression of interband coherence, enhancing net doublon accumulation. Time-frequency analysis uncovers the filling-dependent features of quantum trajectories, manifesting in distinct below-Δ_{\mathrm{Mott}} emission. This doublon-based analysis provides a transparent link between equilibrium spin-charge separation and nonequilibrium strong-field response, and clarifies how dephasing modifies interband coherence and doublon accumulation.
title Tracking doublon-holon dynamics in high-harmonic generation from Mott insulators
topic Optics
url https://arxiv.org/abs/2605.01388