Label-Free Microrefractometry of Interfacial Processes Using Fluorescent Smart Coverslips

Fuente: arXiv
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Bibliographic Details
Main Authors: Klimovsky, Hodaya, Ginsberg, Amitay, Ohorodniichuk, Dmytro, Shehadeh, Maria, Olevsko, Ilya, Byk, Gerardo, Oheim, Martin, Salomon, Adi
Format: Preprint
Published: 2026
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author Klimovsky, Hodaya
Ginsberg, Amitay
Ohorodniichuk, Dmytro
Shehadeh, Maria
Olevsko, Ilya
Byk, Gerardo
Oheim, Martin
Salomon, Adi
author_facet Klimovsky, Hodaya
Ginsberg, Amitay
Ohorodniichuk, Dmytro
Shehadeh, Maria
Olevsko, Ilya
Byk, Gerardo
Oheim, Martin
Salomon, Adi
contents Molecular dipoles near interfaces emit highly directional radiation due to near-field interactions, making surface-bound fluorophores sensitive probes of local physicochemical changes. We introduce smart coverslips, stably coated with uniform, brightly fluorescent nanobead films, that exploit refractive-index-dependent emission shifts for sensitive micro-refractometry in small volumes. Supercritical-angle fluorescence refractometry uses single back-focal-plane images to allow us real-time RI sensing and nanometric thin-film height measurements without the need for multi-angle or multi-wavelength acquisition. Our fast, label-free, and non-invasive approach allows measurements of thin-film properties and monitoring of interfacial dynamics on a standard inverted microscope and is broadly applicable to nanobiophotonics, chemical sensing, and in-situ materials analysis.
format Preprint
id arxiv_https___arxiv_org_abs_2605_01472
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Label-Free Microrefractometry of Interfacial Processes Using Fluorescent Smart Coverslips
Klimovsky, Hodaya
Ginsberg, Amitay
Ohorodniichuk, Dmytro
Shehadeh, Maria
Olevsko, Ilya
Byk, Gerardo
Oheim, Martin
Salomon, Adi
Optics
Quantitative Methods
Molecular dipoles near interfaces emit highly directional radiation due to near-field interactions, making surface-bound fluorophores sensitive probes of local physicochemical changes. We introduce smart coverslips, stably coated with uniform, brightly fluorescent nanobead films, that exploit refractive-index-dependent emission shifts for sensitive micro-refractometry in small volumes. Supercritical-angle fluorescence refractometry uses single back-focal-plane images to allow us real-time RI sensing and nanometric thin-film height measurements without the need for multi-angle or multi-wavelength acquisition. Our fast, label-free, and non-invasive approach allows measurements of thin-film properties and monitoring of interfacial dynamics on a standard inverted microscope and is broadly applicable to nanobiophotonics, chemical sensing, and in-situ materials analysis.
title Label-Free Microrefractometry of Interfacial Processes Using Fluorescent Smart Coverslips
topic Optics
Quantitative Methods
url https://arxiv.org/abs/2605.01472