Metastable MnBi$_2$Te$_4$ enabled by magnetic-field-assisted synthesis

Fuente: arXiv
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Auteurs principaux: Rajbanshi, Abhinna, Zills, G. M., Donald, Alexander M., Duong, Daniel, Graf, David, Hamlin, James J., Meisel, Mark W., Vekhter, I., Shelton, Williams A., Jin, Rongying
Format: Preprint
Publié: 2026
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author Rajbanshi, Abhinna
Zills, G. M.
Donald, Alexander M.
Duong, Daniel
Graf, David
Hamlin, James J.
Meisel, Mark W.
Vekhter, I.
Shelton, Williams A.
Jin, Rongying
author_facet Rajbanshi, Abhinna
Zills, G. M.
Donald, Alexander M.
Duong, Daniel
Graf, David
Hamlin, James J.
Meisel, Mark W.
Vekhter, I.
Shelton, Williams A.
Jin, Rongying
contents Magnetic topological insulators provide a unique platform to explore the interplay between magnetism and topology. MnBi$_2$Te$_4$, known for its A-type antiferromagnetic (AFM) ground state, undergoes a striking transformation when single crystals are grown in an applied magnetic field. Despite retaining the same crystal structure, field-grown MnBi$_2$Te$_4$ exhibits a ferromagnetic (FM) ground state with a Curie temperature of $\sim$ 12.5 K, confirmed by magnetization, magnetic torque, electrical resistivity, and specific heat measurements. First-principles calculations support these findings, revealing that magnetic-field-assisted synthesis can effectively reconfigure the ground-state spin order and thereby modify the material's electronic properties, as reflected in the de Haas-van Alphen oscillation seen in the magnetic torque.
format Preprint
id arxiv_https___arxiv_org_abs_2605_02119
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Metastable MnBi$_2$Te$_4$ enabled by magnetic-field-assisted synthesis
Rajbanshi, Abhinna
Zills, G. M.
Donald, Alexander M.
Duong, Daniel
Graf, David
Hamlin, James J.
Meisel, Mark W.
Vekhter, I.
Shelton, Williams A.
Jin, Rongying
Materials Science
Magnetic topological insulators provide a unique platform to explore the interplay between magnetism and topology. MnBi$_2$Te$_4$, known for its A-type antiferromagnetic (AFM) ground state, undergoes a striking transformation when single crystals are grown in an applied magnetic field. Despite retaining the same crystal structure, field-grown MnBi$_2$Te$_4$ exhibits a ferromagnetic (FM) ground state with a Curie temperature of $\sim$ 12.5 K, confirmed by magnetization, magnetic torque, electrical resistivity, and specific heat measurements. First-principles calculations support these findings, revealing that magnetic-field-assisted synthesis can effectively reconfigure the ground-state spin order and thereby modify the material's electronic properties, as reflected in the de Haas-van Alphen oscillation seen in the magnetic torque.
title Metastable MnBi$_2$Te$_4$ enabled by magnetic-field-assisted synthesis
topic Materials Science
url https://arxiv.org/abs/2605.02119