Understanding the effects of competing spin-pair dephasing pathways in molecular spins

Fuente: arXiv
Saved in:
Bibliographic Details
Main Authors: Krogmeier, Timothy J., Bradley, James, Schlimgen, Anthony W., Head-Marsden, Kade
Format: Preprint
Published: 2026
Subjects:
Online Access:
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1866914528648757248
author Krogmeier, Timothy J.
Bradley, James
Schlimgen, Anthony W.
Head-Marsden, Kade
author_facet Krogmeier, Timothy J.
Bradley, James
Schlimgen, Anthony W.
Head-Marsden, Kade
contents Molecular spins offer promise in emerging quantum technologies such as quantum sensing and computing. At low temperatures, nuclear spin-spin interactions affect electron spin coherence lifetimes through pure dephasing. Nuclear-spin noise can originate from spin pairs within a molecule itself, pairs in a surrounding environment system, or pairs in which one spin is on the molecule and the other in the environment. Improving coherence times requires detailed knowledge of the dominant sources of dephasing. Here, we analyze the decoherence behavior of two molecular qubit candidates with various ligands and in different nuclear-spin containing solvents. We apply an electronic-structure enhanced, non-Markovian perturbative theoretical method to connect experimentally comparable dephasing times to individual spin pairs. This analysis allows the development of a computational workflow to strategically improve coherence lifetimes in spin systems where decoherence is dominated by spin-spin dephasing.
format Preprint
id arxiv_https___arxiv_org_abs_2605_03177
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Understanding the effects of competing spin-pair dephasing pathways in molecular spins
Krogmeier, Timothy J.
Bradley, James
Schlimgen, Anthony W.
Head-Marsden, Kade
Quantum Physics
Molecular spins offer promise in emerging quantum technologies such as quantum sensing and computing. At low temperatures, nuclear spin-spin interactions affect electron spin coherence lifetimes through pure dephasing. Nuclear-spin noise can originate from spin pairs within a molecule itself, pairs in a surrounding environment system, or pairs in which one spin is on the molecule and the other in the environment. Improving coherence times requires detailed knowledge of the dominant sources of dephasing. Here, we analyze the decoherence behavior of two molecular qubit candidates with various ligands and in different nuclear-spin containing solvents. We apply an electronic-structure enhanced, non-Markovian perturbative theoretical method to connect experimentally comparable dephasing times to individual spin pairs. This analysis allows the development of a computational workflow to strategically improve coherence lifetimes in spin systems where decoherence is dominated by spin-spin dephasing.
title Understanding the effects of competing spin-pair dephasing pathways in molecular spins
topic Quantum Physics
url https://arxiv.org/abs/2605.03177