Quantitative cavity-enhanced photothermal dynamics in TMDC-integrated ultrahigh-Q microcavities

Fuente: arXiv
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Autori principali: Kanzawa, Hidetoshi, Sugano, Ryo, Kumazaki, Hajime, Takahashi, Yuta, Watanabe, Shinichi, Fujii, Shun
Natura: Preprint
Pubblicazione: 2026
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author Kanzawa, Hidetoshi
Sugano, Ryo
Kumazaki, Hajime
Takahashi, Yuta
Watanabe, Shinichi
Fujii, Shun
author_facet Kanzawa, Hidetoshi
Sugano, Ryo
Kumazaki, Hajime
Takahashi, Yuta
Watanabe, Shinichi
Fujii, Shun
contents We investigate photothermal effects in monolayer transition metal dichalcogenides (TMDCs) integrated with an ultrahigh-Q silica microcavity. Launching a continuous-wave laser into a cavity resonance enables controlled intracavity heating, allowing direct observation of excitonic photoluminescence (PL) modulation. A distinct redshift of the PL peak energy is observed as the pump wavelength is tuned across resonance. This behavior is quantitatively reproduced by a temperature-dependent bandgap model that combines the Varshni relation with the thermo-optic response of the microcavity, from which the local temperature rise can be estimated. We further find that PL collected through a fiber waveguide exhibits spectral and temporal characteristics markedly different from free-space emission, indicating selective coupling of the microcavity to specific excitonic channels. These results provide a quantitative framework for understanding photothermal effects in TMDC-microcavity hybrid systems and offer a versatile approach for all-optical control and probing of thermal states in integrated nanophotonic devices.
format Preprint
id arxiv_https___arxiv_org_abs_2605_03316
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Quantitative cavity-enhanced photothermal dynamics in TMDC-integrated ultrahigh-Q microcavities
Kanzawa, Hidetoshi
Sugano, Ryo
Kumazaki, Hajime
Takahashi, Yuta
Watanabe, Shinichi
Fujii, Shun
Optics
We investigate photothermal effects in monolayer transition metal dichalcogenides (TMDCs) integrated with an ultrahigh-Q silica microcavity. Launching a continuous-wave laser into a cavity resonance enables controlled intracavity heating, allowing direct observation of excitonic photoluminescence (PL) modulation. A distinct redshift of the PL peak energy is observed as the pump wavelength is tuned across resonance. This behavior is quantitatively reproduced by a temperature-dependent bandgap model that combines the Varshni relation with the thermo-optic response of the microcavity, from which the local temperature rise can be estimated. We further find that PL collected through a fiber waveguide exhibits spectral and temporal characteristics markedly different from free-space emission, indicating selective coupling of the microcavity to specific excitonic channels. These results provide a quantitative framework for understanding photothermal effects in TMDC-microcavity hybrid systems and offer a versatile approach for all-optical control and probing of thermal states in integrated nanophotonic devices.
title Quantitative cavity-enhanced photothermal dynamics in TMDC-integrated ultrahigh-Q microcavities
topic Optics
url https://arxiv.org/abs/2605.03316