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Autores principales: Nemes, Laszlo, Oomens, Jos, Esposito, Vincent J., Boudon, Vincent, Tielens, Alexander G. G. M.
Formato: Preprint
Publicado: 2026
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Acceso en línea:https://arxiv.org/abs/2605.04015
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author Nemes, Laszlo
Oomens, Jos
Esposito, Vincent J.
Boudon, Vincent
Tielens, Alexander G. G. M.
author_facet Nemes, Laszlo
Oomens, Jos
Esposito, Vincent J.
Boudon, Vincent
Tielens, Alexander G. G. M.
contents The largest known molecule in space, C60 , has been detected in its neutral and cationic form through its vibrational, UV-driven fluorescence emission spectrum and its electronic absorption spectrum, respectively. The detection of several polycyclic aromatic hydrocarbon molecules through their pure rotation spectrum in cold, dense, molecular cloud cores suggests that C60 might be present in these environments as well. The low flux of UV pumping photons in molecular cloud cores and the absence of suitably bright background stars, make detection of C60 and its cation through the commonly used methods impractical. As C60 has no permanent dipole moment, its pure rotational transitions are forbidden and its presence must be inferred from the rotational transitions of C60 derivatives with permanent dipole moments. Here, we present a study of the predicted rotational spectrum of protonated C60 that has a sizeable permanent dipole moment. Protonation of C60 reduces the icosahedral symmetry to Cs and results in a dipole moment of about 3.8 Debye. The resulting C60H+ is a closed shell system
format Preprint
id arxiv_https___arxiv_org_abs_2605_04015
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle The Computed Microwave Spectrum of the Protonated Fullerene C60H+
Nemes, Laszlo
Oomens, Jos
Esposito, Vincent J.
Boudon, Vincent
Tielens, Alexander G. G. M.
Astrophysics of Galaxies
The largest known molecule in space, C60 , has been detected in its neutral and cationic form through its vibrational, UV-driven fluorescence emission spectrum and its electronic absorption spectrum, respectively. The detection of several polycyclic aromatic hydrocarbon molecules through their pure rotation spectrum in cold, dense, molecular cloud cores suggests that C60 might be present in these environments as well. The low flux of UV pumping photons in molecular cloud cores and the absence of suitably bright background stars, make detection of C60 and its cation through the commonly used methods impractical. As C60 has no permanent dipole moment, its pure rotational transitions are forbidden and its presence must be inferred from the rotational transitions of C60 derivatives with permanent dipole moments. Here, we present a study of the predicted rotational spectrum of protonated C60 that has a sizeable permanent dipole moment. Protonation of C60 reduces the icosahedral symmetry to Cs and results in a dipole moment of about 3.8 Debye. The resulting C60H+ is a closed shell system
title The Computed Microwave Spectrum of the Protonated Fullerene C60H+
topic Astrophysics of Galaxies
url https://arxiv.org/abs/2605.04015