Correlation-driven tunability of altermagnetism in RuO$_2$

Fuente: arXiv
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Autori principali: Park, Ina, Kim, Dongwook, Lee, Inho, Hong, Jisook, Goh, Beomjoon, Jang, Bo Gyu
Natura: Preprint
Pubblicazione: 2026
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author Park, Ina
Kim, Dongwook
Lee, Inho
Hong, Jisook
Goh, Beomjoon
Jang, Bo Gyu
author_facet Park, Ina
Kim, Dongwook
Lee, Inho
Hong, Jisook
Goh, Beomjoon
Jang, Bo Gyu
contents RuO$_2$ has been regarded as a prototypical candidate for metallic altermagnet, offering a potential platform for high-speed and high-efficiency spintronics. However, the magnetic ground state of RuO$_2$ remains a topic of active debate due to conflicting experimental reports. In this work, we investigate the effect of electron correlations in RuO$_2$ using density functional theory combined with dynamical mean-field theory (DFT+DMFT). In contrast to previous DFT-based studies, DFT+DMFT captures essential dynamical correlation effects, yielding spectral functions and optical conductivities in excellent quantitative agreement with experiments, and further reveals that RuO$_2$ resides in the close vicinity of both the paramagnetic-altermagnetic phase boundary and the itinerant-localized crossover, rendering the magnetic ground state highly susceptible to external perturbations. Indeed, even a minimal compressive strain of $\sim$0.5% is sufficient to drive the system into an altermagnetic phase. These findings elucidate the origin of the conflicting experimental observations and reveal that dynamical correlation effects are the key driving force behind the highly tunable magnetic ground state of RuO$_2$.
format Preprint
id arxiv_https___arxiv_org_abs_2605_13559
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Correlation-driven tunability of altermagnetism in RuO$_2$
Park, Ina
Kim, Dongwook
Lee, Inho
Hong, Jisook
Goh, Beomjoon
Jang, Bo Gyu
Materials Science
Strongly Correlated Electrons
RuO$_2$ has been regarded as a prototypical candidate for metallic altermagnet, offering a potential platform for high-speed and high-efficiency spintronics. However, the magnetic ground state of RuO$_2$ remains a topic of active debate due to conflicting experimental reports. In this work, we investigate the effect of electron correlations in RuO$_2$ using density functional theory combined with dynamical mean-field theory (DFT+DMFT). In contrast to previous DFT-based studies, DFT+DMFT captures essential dynamical correlation effects, yielding spectral functions and optical conductivities in excellent quantitative agreement with experiments, and further reveals that RuO$_2$ resides in the close vicinity of both the paramagnetic-altermagnetic phase boundary and the itinerant-localized crossover, rendering the magnetic ground state highly susceptible to external perturbations. Indeed, even a minimal compressive strain of $\sim$0.5% is sufficient to drive the system into an altermagnetic phase. These findings elucidate the origin of the conflicting experimental observations and reveal that dynamical correlation effects are the key driving force behind the highly tunable magnetic ground state of RuO$_2$.
title Correlation-driven tunability of altermagnetism in RuO$_2$
topic Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2605.13559