p-Wave Orbital Angular Momentum Texture in a Chiral Crystal

Fuente: arXiv
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Auteurs principaux: Oh, Dongjin, Pacella, Chiara, Luo, Xiangyu, Jozwiak, Chris, Bostwick, Aaron, Rotenberg, Eli, Leandersson, Mats, Polley, Craig, Rubio, Angel, Di Sante, Domenico, Comin, Riccardo
Format: Preprint
Publié: 2026
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author Oh, Dongjin
Pacella, Chiara
Luo, Xiangyu
Jozwiak, Chris
Bostwick, Aaron
Rotenberg, Eli
Leandersson, Mats
Polley, Craig
Rubio, Angel
Di Sante, Domenico
Comin, Riccardo
author_facet Oh, Dongjin
Pacella, Chiara
Luo, Xiangyu
Jozwiak, Chris
Bostwick, Aaron
Rotenberg, Eli
Leandersson, Mats
Polley, Craig
Rubio, Angel
Di Sante, Domenico
Comin, Riccardo
contents The spin and orbital angular momentum (SAM and OAM) are conceptually analogous, yet their roles in condensed matter systems have not been often treated on equal footing. While SAM has been extensively explored, OAM has long been regarded as quenched in crystalline environments and thus largely overlooked. Recent experimental and theoretical advances, however, have demonstrated that OAM can drive a variety of novel electronic phenomena, highlighting the importance of probing OAM textures in the electronic band structure. Here, we investigate the momentum-space OAM texture of (TaSe4)2I, a one-dimensional chiral crystal. Using circular-dichroism angle-resolved photoemission spectroscopy (CD-ARPES), we uncover a p-wave OAM texture accompanied by OAM dipole structures. This orbital p-wave texture is intimately connected to, and thus controllable by the chirality of the host lattice. Complementary spin-resolved ARPES measurements and first-principles calculations reveal that the OAM polarization overwhelmingly dominates the low-energy electronic properties of (TaSe4)2I, far exceeding the SAM polarization. These observations represent the experimental verification of a new type of OAM texture in crystalline materials. Most importantly, these findings underscore a promising material platform for spinless orbitronics applications and lay the foundation for realizing multipolar OAM textures-orbital counterparts of the spin texture in unconventional magnets.
format Preprint
id arxiv_https___arxiv_org_abs_2605_15544
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle p-Wave Orbital Angular Momentum Texture in a Chiral Crystal
Oh, Dongjin
Pacella, Chiara
Luo, Xiangyu
Jozwiak, Chris
Bostwick, Aaron
Rotenberg, Eli
Leandersson, Mats
Polley, Craig
Rubio, Angel
Di Sante, Domenico
Comin, Riccardo
Materials Science
The spin and orbital angular momentum (SAM and OAM) are conceptually analogous, yet their roles in condensed matter systems have not been often treated on equal footing. While SAM has been extensively explored, OAM has long been regarded as quenched in crystalline environments and thus largely overlooked. Recent experimental and theoretical advances, however, have demonstrated that OAM can drive a variety of novel electronic phenomena, highlighting the importance of probing OAM textures in the electronic band structure. Here, we investigate the momentum-space OAM texture of (TaSe4)2I, a one-dimensional chiral crystal. Using circular-dichroism angle-resolved photoemission spectroscopy (CD-ARPES), we uncover a p-wave OAM texture accompanied by OAM dipole structures. This orbital p-wave texture is intimately connected to, and thus controllable by the chirality of the host lattice. Complementary spin-resolved ARPES measurements and first-principles calculations reveal that the OAM polarization overwhelmingly dominates the low-energy electronic properties of (TaSe4)2I, far exceeding the SAM polarization. These observations represent the experimental verification of a new type of OAM texture in crystalline materials. Most importantly, these findings underscore a promising material platform for spinless orbitronics applications and lay the foundation for realizing multipolar OAM textures-orbital counterparts of the spin texture in unconventional magnets.
title p-Wave Orbital Angular Momentum Texture in a Chiral Crystal
topic Materials Science
url https://arxiv.org/abs/2605.15544