Interface engineering of the anomalous Hall effect in Ni-based heterostructures

Fuente: arXiv
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Autori principali: Ghosh, Mainak, Yadav, Kusampal, sarkar, Kalyan, Das, Kousik, Mukherjee, Devajyoti, Bhowal, Sayantika
Natura: Preprint
Pubblicazione: 2026
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author Ghosh, Mainak
Yadav, Kusampal
sarkar, Kalyan
Das, Kousik
Mukherjee, Devajyoti
Bhowal, Sayantika
author_facet Ghosh, Mainak
Yadav, Kusampal
sarkar, Kalyan
Das, Kousik
Mukherjee, Devajyoti
Bhowal, Sayantika
contents Using a combined experimental and first-principles theoretical approach, we demonstrate interface engineering of the anomalous Hall effect in Ni-based epitaxial thin-film heterostructures. Ferromagnetic Ni thin films are grown on (001)-oriented single-crystal LaAlO$_3$, SrTiO$_3$, and MgO substrates, which impose different biaxial tensile strains of 0.3%, 0.6%, and 0.8%, respectively. Our room-temperature Hall transport measurements reveal a pronounced substrate-dependent modulation of the anomalous Hall conductivity. Interestingly, our calculations show that strain alone cannot account for the experimentally observed trends. Instead, we identify interfacial inversion-symmetry breaking, which induces Rashba spin-orbit interaction, as the key mechanism governing the anomalous Hall conductivity across different interfaces. Building on this understanding, we further demonstrate both theoretically and experimentally that the anomalous Hall conductivity can be continuously tuned by an external electric field. These findings establish the critical role of substrate-induced interfacial effects in controlling the anomalous Hall effect in engineered heterostructures and provide a viable pathway toward electrically tunable room-temperature spintronic devices.
format Preprint
id arxiv_https___arxiv_org_abs_2605_16936
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Interface engineering of the anomalous Hall effect in Ni-based heterostructures
Ghosh, Mainak
Yadav, Kusampal
sarkar, Kalyan
Das, Kousik
Mukherjee, Devajyoti
Bhowal, Sayantika
Materials Science
Using a combined experimental and first-principles theoretical approach, we demonstrate interface engineering of the anomalous Hall effect in Ni-based epitaxial thin-film heterostructures. Ferromagnetic Ni thin films are grown on (001)-oriented single-crystal LaAlO$_3$, SrTiO$_3$, and MgO substrates, which impose different biaxial tensile strains of 0.3%, 0.6%, and 0.8%, respectively. Our room-temperature Hall transport measurements reveal a pronounced substrate-dependent modulation of the anomalous Hall conductivity. Interestingly, our calculations show that strain alone cannot account for the experimentally observed trends. Instead, we identify interfacial inversion-symmetry breaking, which induces Rashba spin-orbit interaction, as the key mechanism governing the anomalous Hall conductivity across different interfaces. Building on this understanding, we further demonstrate both theoretically and experimentally that the anomalous Hall conductivity can be continuously tuned by an external electric field. These findings establish the critical role of substrate-induced interfacial effects in controlling the anomalous Hall effect in engineered heterostructures and provide a viable pathway toward electrically tunable room-temperature spintronic devices.
title Interface engineering of the anomalous Hall effect in Ni-based heterostructures
topic Materials Science
url https://arxiv.org/abs/2605.16936