Structure of the twist-bend nematic phase with respect to the orientational molecular order of the thioether-linked dimers

Fuente: arXiv
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Main Authors: Kocot, Antoni, Loska, Barbara, Arakawa, Yuki, Merkel, Katarzyna
Format: Preprint
Published: 2026
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author Kocot, Antoni
Loska, Barbara
Arakawa, Yuki
Merkel, Katarzyna
author_facet Kocot, Antoni
Loska, Barbara
Arakawa, Yuki
Merkel, Katarzyna
contents An analysis of the IR absorbance for the segmented functional groups of liquid crystal dimers: mesogen and linker, enabled the orientation order to be determined and information about the dipole interactions in the nematic and twist-bend nematic phases to be obtained. The long axis orientational order increases as the temperature decreases in the nematic phase, although much more slowly than for the classical nematics, and then reverses this trend in the twist-bend nematic phase due to the tilt of the molecules. In the nematic phase, the short axis of the molecule performs an isotropic uniform rotation and has a uniaxial alignment. In the twist-bend nematic phase, however, biaxial ordering occurs and grows significantly in accordance with the helical deformation of the director. Changes in the mean absorbance in the twist-bend nematic phase were observed: a decrease for the longitudinal dipole at the nematic-twist-bend nematic phase transition, thus emphasizing the antiparallel axial interaction of the dipoles, while the absorbance of the transverse dipoles remains unchanged up to 340 K, and then the latter become parallelly correlated.
format Preprint
id arxiv_https___arxiv_org_abs_2605_17523
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Structure of the twist-bend nematic phase with respect to the orientational molecular order of the thioether-linked dimers
Kocot, Antoni
Loska, Barbara
Arakawa, Yuki
Merkel, Katarzyna
Soft Condensed Matter
An analysis of the IR absorbance for the segmented functional groups of liquid crystal dimers: mesogen and linker, enabled the orientation order to be determined and information about the dipole interactions in the nematic and twist-bend nematic phases to be obtained. The long axis orientational order increases as the temperature decreases in the nematic phase, although much more slowly than for the classical nematics, and then reverses this trend in the twist-bend nematic phase due to the tilt of the molecules. In the nematic phase, the short axis of the molecule performs an isotropic uniform rotation and has a uniaxial alignment. In the twist-bend nematic phase, however, biaxial ordering occurs and grows significantly in accordance with the helical deformation of the director. Changes in the mean absorbance in the twist-bend nematic phase were observed: a decrease for the longitudinal dipole at the nematic-twist-bend nematic phase transition, thus emphasizing the antiparallel axial interaction of the dipoles, while the absorbance of the transverse dipoles remains unchanged up to 340 K, and then the latter become parallelly correlated.
title Structure of the twist-bend nematic phase with respect to the orientational molecular order of the thioether-linked dimers
topic Soft Condensed Matter
url https://arxiv.org/abs/2605.17523