Anomalous thermal and elastic properties of an epitaxial NiTi film exhibiting R-phase

Fuente: arXiv
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Auteurs principaux: Repček, Kristýna, Grabec, Tomáš, Mareš, David, Stoklasová, Pavla, Sedlák, Petr, Kušnír, Jakub, Veřtát, Petr, Heczko, Oleg, Fähler, Sebastian, Lünser, Klara, Seiner, H.
Format: Preprint
Publié: 2026
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author Repček, Kristýna
Grabec, Tomáš
Mareš, David
Stoklasová, Pavla
Sedlák, Petr
Kušnír, Jakub
Veřtát, Petr
Heczko, Oleg
Fähler, Sebastian
Lünser, Klara
Seiner, H.
author_facet Repček, Kristýna
Grabec, Tomáš
Mareš, David
Stoklasová, Pavla
Sedlák, Petr
Kušnír, Jakub
Veřtát, Petr
Heczko, Oleg
Fähler, Sebastian
Lünser, Klara
Seiner, H.
contents Shape memory alloys like NiTi are at the core of emerging thermal management applications, including elastocaloric refrigeration, thermoelastic harvesting, and latent heat storage. Most of these applications benefit from a small scale due to the accelerated heat exchange, but obtaining precise functional properties of films is challenging. Here we demonstrate that transient grating spectroscopy (TGS) enables characterization of elastic coefficients and thermal diffusivity of a 3 $μ$m thick epitaxial NiTi film during a thermally induced phase transformation. The in-situ measurement of a complete austenite$\rightarrow$R-phase$\rightarrow$martensite$\rightarrow$austenite temperature cycle reveals that the elastic properties exhibit a crossover of the shear moduli (from $c^\prime < c_{44}$ in austenite to $c^\prime > c_{44}$ in martensite) and that the thermal diffusivity changes by 450 $\%$ between the R-phase and austenite. This dramatic change, together with the absence of hysteresis between the R-phase and austenite, makes NiTi a promising material candidate for thermal switches. The results indicate that the change in thermal diffusivity originates from an anomalous heat capacity of the R-phase. Furthermore, our TGS study provides temperature-dependent thermal and elastic properties required for simulating thermal management microsystems using this material.
format Preprint
id arxiv_https___arxiv_org_abs_2605_17553
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Anomalous thermal and elastic properties of an epitaxial NiTi film exhibiting R-phase
Repček, Kristýna
Grabec, Tomáš
Mareš, David
Stoklasová, Pavla
Sedlák, Petr
Kušnír, Jakub
Veřtát, Petr
Heczko, Oleg
Fähler, Sebastian
Lünser, Klara
Seiner, H.
Materials Science
Shape memory alloys like NiTi are at the core of emerging thermal management applications, including elastocaloric refrigeration, thermoelastic harvesting, and latent heat storage. Most of these applications benefit from a small scale due to the accelerated heat exchange, but obtaining precise functional properties of films is challenging. Here we demonstrate that transient grating spectroscopy (TGS) enables characterization of elastic coefficients and thermal diffusivity of a 3 $μ$m thick epitaxial NiTi film during a thermally induced phase transformation. The in-situ measurement of a complete austenite$\rightarrow$R-phase$\rightarrow$martensite$\rightarrow$austenite temperature cycle reveals that the elastic properties exhibit a crossover of the shear moduli (from $c^\prime < c_{44}$ in austenite to $c^\prime > c_{44}$ in martensite) and that the thermal diffusivity changes by 450 $\%$ between the R-phase and austenite. This dramatic change, together with the absence of hysteresis between the R-phase and austenite, makes NiTi a promising material candidate for thermal switches. The results indicate that the change in thermal diffusivity originates from an anomalous heat capacity of the R-phase. Furthermore, our TGS study provides temperature-dependent thermal and elastic properties required for simulating thermal management microsystems using this material.
title Anomalous thermal and elastic properties of an epitaxial NiTi film exhibiting R-phase
topic Materials Science
url https://arxiv.org/abs/2605.17553