Superconducting PdTe Thin Film Via Topotactic Transformation, Toward Topological Superconductors

Fuente: arXiv
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Auteurs principaux: Yi, Hee Taek, Ge, Min, Xie, Renjie, Stoddard, Colby J., Yi, David H., Yuan, Xiaoyu, Yao, Xiong, Oh, Seongshik
Format: Preprint
Publié: 2026
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author Yi, Hee Taek
Ge, Min
Xie, Renjie
Stoddard, Colby J.
Yi, David H.
Yuan, Xiaoyu
Yao, Xiong
Oh, Seongshik
author_facet Yi, Hee Taek
Ge, Min
Xie, Renjie
Stoddard, Colby J.
Yi, David H.
Yuan, Xiaoyu
Yao, Xiong
Oh, Seongshik
contents Topological superconductors (TSCs) hosting Majorana zero modes (MZMs) offer a pathway to fault-tolerant quantum computation. PdTe is a promising TSC candidate due to its topological surface states and a reasonable superconducting critical temperature of ~4.5 K. However, it has been challenging to grow PdTe thin films with bulk-like superconducting properties. Here, we show that high-quality, superconducting PdTe thin films can be grown using molecular beam epitaxy (MBE). The films exhibit a sharp superconducting transition (T_onset = 4.43 K with transition width of 0.06 K), comparable to that of bulk crystals. This was made possible via a topotactic transformation from a PdTe_2 buffer layer to a PdTe phase by growing Pd on top under Te-deficient conditions. Structural and transport analyses confirm the NiAs-type structure of PdTe, as well as its two-dimensional superconducting behavior and excellent air stability. These findings suggest that the MBE-grown PdTe films and their heterostructures are a promising platform for topological superconductivity and Majorana physics.
format Preprint
id arxiv_https___arxiv_org_abs_2605_20437
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Superconducting PdTe Thin Film Via Topotactic Transformation, Toward Topological Superconductors
Yi, Hee Taek
Ge, Min
Xie, Renjie
Stoddard, Colby J.
Yi, David H.
Yuan, Xiaoyu
Yao, Xiong
Oh, Seongshik
Superconductivity
Materials Science
Topological superconductors (TSCs) hosting Majorana zero modes (MZMs) offer a pathway to fault-tolerant quantum computation. PdTe is a promising TSC candidate due to its topological surface states and a reasonable superconducting critical temperature of ~4.5 K. However, it has been challenging to grow PdTe thin films with bulk-like superconducting properties. Here, we show that high-quality, superconducting PdTe thin films can be grown using molecular beam epitaxy (MBE). The films exhibit a sharp superconducting transition (T_onset = 4.43 K with transition width of 0.06 K), comparable to that of bulk crystals. This was made possible via a topotactic transformation from a PdTe_2 buffer layer to a PdTe phase by growing Pd on top under Te-deficient conditions. Structural and transport analyses confirm the NiAs-type structure of PdTe, as well as its two-dimensional superconducting behavior and excellent air stability. These findings suggest that the MBE-grown PdTe films and their heterostructures are a promising platform for topological superconductivity and Majorana physics.
title Superconducting PdTe Thin Film Via Topotactic Transformation, Toward Topological Superconductors
topic Superconductivity
Materials Science
url https://arxiv.org/abs/2605.20437