Ultrafast excitation of Bloch plasmon polaritons in hyperbolic metamaterials with an extreme ultra-violet transient grating

Fuente: arXiv
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Autori principali: Tapani, Tlek, Kempf, Hannes, Pancaldi, Matteo, Foglia, Laura, Pedersoli, Emanuele, Totani, Roberta, Valerio, Adriana, Mincigrucci, Riccardo, Nikolov, Ivaylo, Danailov, Miltcho B., De Andrés, Aitor, Krahne, Roman, Vavassori, Paolo, Bencivenga, Filippo, Capotondi, Flavio, Garoli, Denis, Maccaferri, Nicolò
Natura: Preprint
Pubblicazione: 2026
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author Tapani, Tlek
Kempf, Hannes
Pancaldi, Matteo
Foglia, Laura
Pedersoli, Emanuele
Totani, Roberta
Valerio, Adriana
Mincigrucci, Riccardo
Nikolov, Ivaylo
Danailov, Miltcho B.
De Andrés, Aitor
Krahne, Roman
Vavassori, Paolo
Bencivenga, Filippo
Capotondi, Flavio
Garoli, Denis
Maccaferri, Nicolò
author_facet Tapani, Tlek
Kempf, Hannes
Pancaldi, Matteo
Foglia, Laura
Pedersoli, Emanuele
Totani, Roberta
Valerio, Adriana
Mincigrucci, Riccardo
Nikolov, Ivaylo
Danailov, Miltcho B.
De Andrés, Aitor
Krahne, Roman
Vavassori, Paolo
Bencivenga, Filippo
Capotondi, Flavio
Garoli, Denis
Maccaferri, Nicolò
contents Manipulating materials properties with light drives advances in materials science and photonics. Hyperbolic metamaterials are promising candidates as next-generation quantum optical media. They support Bloch plasmon polaritons, which are characterized by potentially infinite wave-vectors and long lifetimes, but cannot be excited through direct light illumination due to momentum mismatch. Here, we experimentally show that a transient grating, formed via interference of fully coherent seeded free-electron laser pulses in a thin insulator film, enables the excitation of Bloch plasmon polaritons in an underlying hyperbolic metamaterial. Finite element simulations confirm the role of the transient grating in facilitating phase-matching and mode excitation. Our findings demonstrate a route to spatiotemporally excite Bloch plasmon polaritons modes, offering an alternative to permanently nanostructured gratings and potentially enabling ultrafast control of optical modes excitation.
format Preprint
id arxiv_https___arxiv_org_abs_2605_20513
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Ultrafast excitation of Bloch plasmon polaritons in hyperbolic metamaterials with an extreme ultra-violet transient grating
Tapani, Tlek
Kempf, Hannes
Pancaldi, Matteo
Foglia, Laura
Pedersoli, Emanuele
Totani, Roberta
Valerio, Adriana
Mincigrucci, Riccardo
Nikolov, Ivaylo
Danailov, Miltcho B.
De Andrés, Aitor
Krahne, Roman
Vavassori, Paolo
Bencivenga, Filippo
Capotondi, Flavio
Garoli, Denis
Maccaferri, Nicolò
Optics
Materials Science
Manipulating materials properties with light drives advances in materials science and photonics. Hyperbolic metamaterials are promising candidates as next-generation quantum optical media. They support Bloch plasmon polaritons, which are characterized by potentially infinite wave-vectors and long lifetimes, but cannot be excited through direct light illumination due to momentum mismatch. Here, we experimentally show that a transient grating, formed via interference of fully coherent seeded free-electron laser pulses in a thin insulator film, enables the excitation of Bloch plasmon polaritons in an underlying hyperbolic metamaterial. Finite element simulations confirm the role of the transient grating in facilitating phase-matching and mode excitation. Our findings demonstrate a route to spatiotemporally excite Bloch plasmon polaritons modes, offering an alternative to permanently nanostructured gratings and potentially enabling ultrafast control of optical modes excitation.
title Ultrafast excitation of Bloch plasmon polaritons in hyperbolic metamaterials with an extreme ultra-violet transient grating
topic Optics
Materials Science
url https://arxiv.org/abs/2605.20513