Tuning the low-energy band structure in twisted bilayer WSe2

Fuente: arXiv
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Autori principali: Vu, T. -H. -Y., Clark, O. J., Jo, N. H., Blyth, J., Li, Q., Jozwiak, C., Bostwick, A., Muir, J. B., Jia, L., Davis, J. A., Di Bernardo, I., Cabo, A. Grubisic, Xing, K., Zhao, W., Ryu, S. H., Lee, S. H., Mao, Z., Watanabe, K., Taniguchi, T., Chambers, B. A., Harmer, S. L., Rotenberg, E., Fuhrer, M. S., Edmonds, M. T.
Natura: Preprint
Pubblicazione: 2026
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author Vu, T. -H. -Y.
Clark, O. J.
Jo, N. H.
Blyth, J.
Li, Q.
Jozwiak, C.
Bostwick, A.
Muir, J. B.
Jia, L.
Davis, J. A.
Di Bernardo, I.
Cabo, A. Grubisic
Xing, K.
Zhao, W.
Ryu, S. H.
Lee, S. H.
Mao, Z.
Watanabe, K.
Taniguchi, T.
Chambers, B. A.
Harmer, S. L.
Rotenberg, E.
Fuhrer, M. S.
Edmonds, M. T.
author_facet Vu, T. -H. -Y.
Clark, O. J.
Jo, N. H.
Blyth, J.
Li, Q.
Jozwiak, C.
Bostwick, A.
Muir, J. B.
Jia, L.
Davis, J. A.
Di Bernardo, I.
Cabo, A. Grubisic
Xing, K.
Zhao, W.
Ryu, S. H.
Lee, S. H.
Mao, Z.
Watanabe, K.
Taniguchi, T.
Chambers, B. A.
Harmer, S. L.
Rotenberg, E.
Fuhrer, M. S.
Edmonds, M. T.
contents Tuning the electronic structures of two-dimensional (2D) material-based heterostructures is of crucial importance for their use in functional next-generation electronics. Here, through angle-resolved photoemission spectroscopy with nanoscale spatial resolution (nano-ARPES), we systematically track the evolution of the near-Fermi-level electronic structure of bilayer WSe2 over a large range of twist angle. While the momentum positioning of the valence band maxima is independent of twist angle, we find that the energetic separation between the hole bands at the K point of the Brillouin zone and the higher binding-energy hole band at Γ can be varied in excess of 100 meV. We explore the mechanisms underpinning this evolution and discuss the implications for tuning both the size of the band gaps, and the efficiency of the spin-dependent electron-phonon coupling channels in homobilayer transition metal dichalcogenide devices.
format Preprint
id arxiv_https___arxiv_org_abs_2605_20671
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Tuning the low-energy band structure in twisted bilayer WSe2
Vu, T. -H. -Y.
Clark, O. J.
Jo, N. H.
Blyth, J.
Li, Q.
Jozwiak, C.
Bostwick, A.
Muir, J. B.
Jia, L.
Davis, J. A.
Di Bernardo, I.
Cabo, A. Grubisic
Xing, K.
Zhao, W.
Ryu, S. H.
Lee, S. H.
Mao, Z.
Watanabe, K.
Taniguchi, T.
Chambers, B. A.
Harmer, S. L.
Rotenberg, E.
Fuhrer, M. S.
Edmonds, M. T.
Materials Science
Mesoscale and Nanoscale Physics
Tuning the electronic structures of two-dimensional (2D) material-based heterostructures is of crucial importance for their use in functional next-generation electronics. Here, through angle-resolved photoemission spectroscopy with nanoscale spatial resolution (nano-ARPES), we systematically track the evolution of the near-Fermi-level electronic structure of bilayer WSe2 over a large range of twist angle. While the momentum positioning of the valence band maxima is independent of twist angle, we find that the energetic separation between the hole bands at the K point of the Brillouin zone and the higher binding-energy hole band at Γ can be varied in excess of 100 meV. We explore the mechanisms underpinning this evolution and discuss the implications for tuning both the size of the band gaps, and the efficiency of the spin-dependent electron-phonon coupling channels in homobilayer transition metal dichalcogenide devices.
title Tuning the low-energy band structure in twisted bilayer WSe2
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2605.20671