Pulse-Driven Reconfiguration of Fractional Polar Topology in Zr-Substituted Barium Titanate
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arXiv
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| Natura: | Preprint |
| Pubblicazione: |
2026
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| _version_ | 1866918514680397824 |
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| author | Mayer, Florian |
| author_facet | Mayer, Florian |
| contents | Polar topological textures in ferroelectrics can host internal structure beyond a single integer topological charge. Here, effective-Hamiltonian molecular-dynamics simulations are used to examine whether such internal fractional topology can be reconfigured by local electric excitation in ordered 12.5% Zr-substituted barium titanate. Chemical doubling along the polar axis stabilizes a coupled nanodomain texture consisting of alternating Q = -2 antiskyrmionic and Q = +4 skyrmionic slices, in which the local topological charge fragments into six -1/3 and six +2/3 localized contributions, denoted here as topological quarks, separated by Bloch-point-like singular conversion regions. Picosecond local electric-field pulses applied to selected vortex-core columns drive reconfiguration of the internal dipolar texture of a 2.6 nm nanodomain. Under a binary pulse-mask protocol addressing the six vortex cores, all 64 masks lead, within the chosen low-temperature simulation protocol, to distinct relaxed metastable configurations. The switching calculations are performed in a cryogenic regime, and the programmed states remain stable over at least 1 ns of field-free evolution on the simulation timescale. The resulting configurations are distinguishable both by sector-resolved topological fingerprints and by their real-space polarization fields. These results provide a computational proof of concept that fractional polar topology in a ferroelectric nanodomain can be locally reconfigured by ultrafast electric excitation and used as a multistate configurational degree of freedom in an idealized low-temperature setting. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2605_21368 |
| institution | arXiv |
| publishDate | 2026 |
| record_format | arxiv |
| spellingShingle | Pulse-Driven Reconfiguration of Fractional Polar Topology in Zr-Substituted Barium Titanate Mayer, Florian Materials Science Mesoscale and Nanoscale Physics Polar topological textures in ferroelectrics can host internal structure beyond a single integer topological charge. Here, effective-Hamiltonian molecular-dynamics simulations are used to examine whether such internal fractional topology can be reconfigured by local electric excitation in ordered 12.5% Zr-substituted barium titanate. Chemical doubling along the polar axis stabilizes a coupled nanodomain texture consisting of alternating Q = -2 antiskyrmionic and Q = +4 skyrmionic slices, in which the local topological charge fragments into six -1/3 and six +2/3 localized contributions, denoted here as topological quarks, separated by Bloch-point-like singular conversion regions. Picosecond local electric-field pulses applied to selected vortex-core columns drive reconfiguration of the internal dipolar texture of a 2.6 nm nanodomain. Under a binary pulse-mask protocol addressing the six vortex cores, all 64 masks lead, within the chosen low-temperature simulation protocol, to distinct relaxed metastable configurations. The switching calculations are performed in a cryogenic regime, and the programmed states remain stable over at least 1 ns of field-free evolution on the simulation timescale. The resulting configurations are distinguishable both by sector-resolved topological fingerprints and by their real-space polarization fields. These results provide a computational proof of concept that fractional polar topology in a ferroelectric nanodomain can be locally reconfigured by ultrafast electric excitation and used as a multistate configurational degree of freedom in an idealized low-temperature setting. |
| title | Pulse-Driven Reconfiguration of Fractional Polar Topology in Zr-Substituted Barium Titanate |
| topic | Materials Science Mesoscale and Nanoscale Physics |
| url | https://arxiv.org/abs/2605.21368 |