Equilibrium Stabilization of a Hidden Phase Like Metallic State in 1T-TaS2

Fuente: arXiv
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Main Authors: Yilmaz, Turgut, Rajapitamahuni, Anil, Park, Suji, Jang, Houk, Kundu, Asish K., Vescovo, Elio
Format: Preprint
Published: 2026
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author Yilmaz, Turgut
Rajapitamahuni, Anil
Park, Suji
Jang, Houk
Kundu, Asish K.
Vescovo, Elio
author_facet Yilmaz, Turgut
Rajapitamahuni, Anil
Park, Suji
Jang, Houk
Kundu, Asish K.
Vescovo, Elio
contents Electronic phases that lie outside the equilibrium ground state offer a route to explore competing configurations in correlated materials. In 1T-TaS2, ultrafast excitation accesses a metallic hidden phase that is distinct from the commensurate insulating ground state. Here we use angle-resolved photoemission spectroscopy to show that an equivalent electronic configuration is stabilized in exfoliated intermediate-thickness 1T-TaS2 flakes, where it persists up to room temperature before evolving through a different sequence of electronic transitions. This equilibrium hidden-phase-like state hosts a metallic band with finite Fermi-level spectral weight while retaining the characteristic hybridization gaps associated with the star-of-David band folding. These results establish a platform for controlling competing electronic states in layered materials, with implications for both quantum science and phase change technologies.
format Preprint
id arxiv_https___arxiv_org_abs_2605_22292
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Equilibrium Stabilization of a Hidden Phase Like Metallic State in 1T-TaS2
Yilmaz, Turgut
Rajapitamahuni, Anil
Park, Suji
Jang, Houk
Kundu, Asish K.
Vescovo, Elio
Strongly Correlated Electrons
Materials Science
Electronic phases that lie outside the equilibrium ground state offer a route to explore competing configurations in correlated materials. In 1T-TaS2, ultrafast excitation accesses a metallic hidden phase that is distinct from the commensurate insulating ground state. Here we use angle-resolved photoemission spectroscopy to show that an equivalent electronic configuration is stabilized in exfoliated intermediate-thickness 1T-TaS2 flakes, where it persists up to room temperature before evolving through a different sequence of electronic transitions. This equilibrium hidden-phase-like state hosts a metallic band with finite Fermi-level spectral weight while retaining the characteristic hybridization gaps associated with the star-of-David band folding. These results establish a platform for controlling competing electronic states in layered materials, with implications for both quantum science and phase change technologies.
title Equilibrium Stabilization of a Hidden Phase Like Metallic State in 1T-TaS2
topic Strongly Correlated Electrons
Materials Science
url https://arxiv.org/abs/2605.22292