Tuning J$_1$-J$_2$ in Quasi-2D Triangular Lattice Antiferromagnet $α$-SrCr$_2$O$_4$ via Uniaxial Pressure
Fuente:
arXiv
Saved in:
| Main Authors: | , , , , |
|---|---|
| Format: | Preprint |
| Published: |
2026
|
| Subjects: | |
| Online Access: | |
| Tags: |
Add Tag
No Tags, Be the first to tag this record!
|
| _version_ | 1866910247481769984 |
|---|---|
| author | Victorin, Jazzmin Ghosh, Shreenanda Koohpayeh, Seyed Lygouras, Chris Drichko, Natalia |
| author_facet | Victorin, Jazzmin Ghosh, Shreenanda Koohpayeh, Seyed Lygouras, Chris Drichko, Natalia |
| contents | Triangular lattice antiferromagnets first attracted attention as a frustrated magnetic lattice which can serve as a platform to realize the resonating valence bond state. While the triangular lattice itself was shown to support classical 120 degree order, many theoretical phase diagrams suggest a quantum spin liquid state within a small range of parameters. One possible avenue to achieve such a state is to tune the anisotropy of the triangular lattice antiferromagnet by applying uniaxial pressure. This motivated our Raman scattering study of quasi-two-dimensional antiferromagnet $α$-SrCr$_2$O$_4$ under applied uniaxial pressure. Under ambient conditions, $α$-SrCr$_2$O$_4$ develops long-range helical magnetic order below T$_N$ = 43 K. We identify two-magnon excitations associated with this long-range antiferromagnetic order below T$_N$ at 15.5 meV and 40 meV by comparison with spin wave calculations. We observe the two features from the two-magnon excitation shift away from (towards) each other under applied tensile (compressive) pressure, indicating a decrease (increase) in anisotropy. Raman active phonons show a shift to higher (lower) frequencies under applied compressive (tensile) pressure, indicating efficient transmission of pressure and tuning of the lattice. We show spin wave and two-magnon density of states calculations under uniaxial pressure are consistent with our experimental results. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2605_23133 |
| institution | arXiv |
| publishDate | 2026 |
| record_format | arxiv |
| spellingShingle | Tuning J$_1$-J$_2$ in Quasi-2D Triangular Lattice Antiferromagnet $α$-SrCr$_2$O$_4$ via Uniaxial Pressure Victorin, Jazzmin Ghosh, Shreenanda Koohpayeh, Seyed Lygouras, Chris Drichko, Natalia Strongly Correlated Electrons Triangular lattice antiferromagnets first attracted attention as a frustrated magnetic lattice which can serve as a platform to realize the resonating valence bond state. While the triangular lattice itself was shown to support classical 120 degree order, many theoretical phase diagrams suggest a quantum spin liquid state within a small range of parameters. One possible avenue to achieve such a state is to tune the anisotropy of the triangular lattice antiferromagnet by applying uniaxial pressure. This motivated our Raman scattering study of quasi-two-dimensional antiferromagnet $α$-SrCr$_2$O$_4$ under applied uniaxial pressure. Under ambient conditions, $α$-SrCr$_2$O$_4$ develops long-range helical magnetic order below T$_N$ = 43 K. We identify two-magnon excitations associated with this long-range antiferromagnetic order below T$_N$ at 15.5 meV and 40 meV by comparison with spin wave calculations. We observe the two features from the two-magnon excitation shift away from (towards) each other under applied tensile (compressive) pressure, indicating a decrease (increase) in anisotropy. Raman active phonons show a shift to higher (lower) frequencies under applied compressive (tensile) pressure, indicating efficient transmission of pressure and tuning of the lattice. We show spin wave and two-magnon density of states calculations under uniaxial pressure are consistent with our experimental results. |
| title | Tuning J$_1$-J$_2$ in Quasi-2D Triangular Lattice Antiferromagnet $α$-SrCr$_2$O$_4$ via Uniaxial Pressure |
| topic | Strongly Correlated Electrons |
| url | https://arxiv.org/abs/2605.23133 |