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Autores principales: van Essen, Pieter J., Cárdenas, Aday, Silva, Rui E. F., Galán, Álvaro Jiménez, Kraus, Peter M.
Formato: Preprint
Publicado: 2026
Materias:
Acceso en línea:https://arxiv.org/abs/2605.23534
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author van Essen, Pieter J.
Cárdenas, Aday
Silva, Rui E. F.
Galán, Álvaro Jiménez
Kraus, Peter M.
author_facet van Essen, Pieter J.
Cárdenas, Aday
Silva, Rui E. F.
Galán, Álvaro Jiménez
Kraus, Peter M.
contents Ultrafast all-optical control of light emission is a central goal of extreme nonlinear optics, with implications for compact short-wavelength sources, petahertz optoelectronics, and label-free superresolution microscopy. High-harmonic generation in solids is a particularly attractive platform for this goal because it is highly sensitive to both the driving field and the material response, yet a generally applicable framework for controlling harmonic emission has remained elusive. Here, we demonstrate programmable control of high-harmonic emission in solids and show that it can be quantitatively described within a photon-pathway framework. We find that harmonic emission can be suppressed or enhanced by tuning two experimentally accessible quantities: the effective nonlinear order and the intrinsic emission phase. Across a wide range of semiconductors and dielectrics, this approach unifies parametric and non-parametric modulation, explains distinct delay-dependent spectral responses, and reproduces strong suppression, enhancement, and higher-order pathway revivals. Semiconductor Bloch equation simulations support the model and provide a complementary time-domain picture in which the control field reshapes the interference of sub-cycle emission events. These results establish high-harmonic generation in solids as a programmable emission process and provide a general route towards ultrafast optical switching, compact coherent short-wavelength sources, and label-free attosecond super-resolution microscopy.
format Preprint
id arxiv_https___arxiv_org_abs_2605_23534
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Programmable high-harmonic emission in solids through photon pathways
van Essen, Pieter J.
Cárdenas, Aday
Silva, Rui E. F.
Galán, Álvaro Jiménez
Kraus, Peter M.
Optics
Ultrafast all-optical control of light emission is a central goal of extreme nonlinear optics, with implications for compact short-wavelength sources, petahertz optoelectronics, and label-free superresolution microscopy. High-harmonic generation in solids is a particularly attractive platform for this goal because it is highly sensitive to both the driving field and the material response, yet a generally applicable framework for controlling harmonic emission has remained elusive. Here, we demonstrate programmable control of high-harmonic emission in solids and show that it can be quantitatively described within a photon-pathway framework. We find that harmonic emission can be suppressed or enhanced by tuning two experimentally accessible quantities: the effective nonlinear order and the intrinsic emission phase. Across a wide range of semiconductors and dielectrics, this approach unifies parametric and non-parametric modulation, explains distinct delay-dependent spectral responses, and reproduces strong suppression, enhancement, and higher-order pathway revivals. Semiconductor Bloch equation simulations support the model and provide a complementary time-domain picture in which the control field reshapes the interference of sub-cycle emission events. These results establish high-harmonic generation in solids as a programmable emission process and provide a general route towards ultrafast optical switching, compact coherent short-wavelength sources, and label-free attosecond super-resolution microscopy.
title Programmable high-harmonic emission in solids through photon pathways
topic Optics
url https://arxiv.org/abs/2605.23534