_version_ 1866918523397210112
author Hao, Zhanyang
Sheng, Haohao
Ma, Wanru
Zheng, Wengen
Cai, Yongqing
Xie, Zijuan
Cheng, Wanlin
Liang, Zuowei
Xie, Wu
Zhao, Wenjuan
Liu, Chen
Su, Zhibin
Lin, Junhao
Wu, Liusuo
Liu, Zhengtai
Ye, Mao
Dai, Ji
Tallarida, Massimo
Cui, Shengtao
Kumar, Yogendra
Shimada, Kenya
Ozawa, Kenichi
Torii, Shuki
Mori, Kazuhiro
Xie, Yue
Deng, Junze
Wang, Jiaou
Zhu, Xuetao
Guo, Jiandong
Mei, Jiawei
Wang, Zhenyu
Chen, Xianhui
Miao, Ping
Wang, Zhijun
Chen, Chaoyu
author_facet Hao, Zhanyang
Sheng, Haohao
Ma, Wanru
Zheng, Wengen
Cai, Yongqing
Xie, Zijuan
Cheng, Wanlin
Liang, Zuowei
Xie, Wu
Zhao, Wenjuan
Liu, Chen
Su, Zhibin
Lin, Junhao
Wu, Liusuo
Liu, Zhengtai
Ye, Mao
Dai, Ji
Tallarida, Massimo
Cui, Shengtao
Kumar, Yogendra
Shimada, Kenya
Ozawa, Kenichi
Torii, Shuki
Mori, Kazuhiro
Xie, Yue
Deng, Junze
Wang, Jiaou
Zhu, Xuetao
Guo, Jiandong
Mei, Jiawei
Wang, Zhenyu
Chen, Xianhui
Miao, Ping
Wang, Zhijun
Chen, Chaoyu
contents Orbital order describes a quantum state where occupied orbitals line up in a periodic pattern. While orbital physics plays a fundamental and universal role in strongly correlated electron systems, the existence and particularly the band structure fingerprint of orbital order remain a long-standing mystery. Here, we report the discovery of rare earth 5d-orbital order developed by the surface states of intermetallic compound Tb2CoAl4Ge2. Angle-resolved photoemission spectroscopy reveals characteristic nematic features like Fermi surface deformation and band split. These experimental observations can be described by a ferro-orbital order term in the mean-field Hamiltonian. The structural and magnetic origin of such order is excluded by systematic high-resolution neutron powder diffraction and scanning tunnelling microscopy measurements. Our results provide strong evidence for a pure surface orbital order scenario avoiding complications from structural distortion as in colossal magnetoresistance manganites, magnetic order as in iron-based superconductors, and charge transfer p-orbital order in cuprates.
format Preprint
id arxiv_https___arxiv_org_abs_2605_26426
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Surface d-orbital order in intermetallic compound
Hao, Zhanyang
Sheng, Haohao
Ma, Wanru
Zheng, Wengen
Cai, Yongqing
Xie, Zijuan
Cheng, Wanlin
Liang, Zuowei
Xie, Wu
Zhao, Wenjuan
Liu, Chen
Su, Zhibin
Lin, Junhao
Wu, Liusuo
Liu, Zhengtai
Ye, Mao
Dai, Ji
Tallarida, Massimo
Cui, Shengtao
Kumar, Yogendra
Shimada, Kenya
Ozawa, Kenichi
Torii, Shuki
Mori, Kazuhiro
Xie, Yue
Deng, Junze
Wang, Jiaou
Zhu, Xuetao
Guo, Jiandong
Mei, Jiawei
Wang, Zhenyu
Chen, Xianhui
Miao, Ping
Wang, Zhijun
Chen, Chaoyu
Strongly Correlated Electrons
Orbital order describes a quantum state where occupied orbitals line up in a periodic pattern. While orbital physics plays a fundamental and universal role in strongly correlated electron systems, the existence and particularly the band structure fingerprint of orbital order remain a long-standing mystery. Here, we report the discovery of rare earth 5d-orbital order developed by the surface states of intermetallic compound Tb2CoAl4Ge2. Angle-resolved photoemission spectroscopy reveals characteristic nematic features like Fermi surface deformation and band split. These experimental observations can be described by a ferro-orbital order term in the mean-field Hamiltonian. The structural and magnetic origin of such order is excluded by systematic high-resolution neutron powder diffraction and scanning tunnelling microscopy measurements. Our results provide strong evidence for a pure surface orbital order scenario avoiding complications from structural distortion as in colossal magnetoresistance manganites, magnetic order as in iron-based superconductors, and charge transfer p-orbital order in cuprates.
title Surface d-orbital order in intermetallic compound
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2605.26426