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Bibliographic Details
Main Authors: Hiller, Han S., Parakh, Pranav, Aronson, Samuel H., Maeda, Kenji, Lao, Di, Stewart, Julian, She, Zengde, Wang, Jierong, Xu, Xiaodong, Heinz, Tony, Lev, Benjamin L.
Format: Preprint
Published: 2026
Subjects:
Online Access:https://arxiv.org/abs/2605.28815
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Table of Contents:
  • Two-dimensional van der Waals materials exhibit a variety of correlated electron phases, and optical driving offers a promising route toward manipulating them. For example, cavity-enhanced, continuous-wave (CW) Raman excitation has been suggested as a way to coherently and superradiantly populate phonons or charge density waves via material excitons. A steady-state phonon population may be sustained with sufficiently strong electron-phonon coupling to drive novel collective response. We describe an apparatus built to meet the requirements of such an experimental program: Namely, an ultrahigh-vacuum system housing a length-tunable confocal Fabry-Pérot cavity with an intracavity sample, both cryogenically cooled and stabilized against vibrations. A four-axis nanopositioner aligns the sample and supports electrical leads for sample carrier density modulation and transport measurements. Transmission through the multimode cavity enables in situ sample imaging for alignment; the sample is a transition metal dichalcogenide in this work. Operating near the confocal geometry concentrates the optical field into a localized supermode that substantially enhances light-matter coupling. This enhancement is preserved despite the millimeter-scale cavity length, which provides room for sample alignment and exchange.