Magnetic domains reconfiguration on the Fe3O4(110) surface across the Verwey transition by Spin-Polarized Low-Energy Electron Microscopy

Fuente: arXiv
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Main Authors: Gutiérrez-Cuesta, C., Mandziak, A., Prieto, J. E., Nita, P., Mascaraque, A., Choudhry, U., Turner, J., Stibor, A., de la Figuera, J.
Format: Preprint
Published: 2026
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author Gutiérrez-Cuesta, C.
Mandziak, A.
Prieto, J. E.
Nita, P.
Mascaraque, A.
Choudhry, U.
Turner, J.
Stibor, A.
de la Figuera, J.
author_facet Gutiérrez-Cuesta, C.
Mandziak, A.
Prieto, J. E.
Nita, P.
Mascaraque, A.
Choudhry, U.
Turner, J.
Stibor, A.
de la Figuera, J.
contents We have studied the (110) surface of Fe$_3$O$_4$ single crystals by means of spin-polarized low-energy electron microscopy (SPLEEM). After preparation by sputtering and annealing a well defined reconstructed surface was achieved, composed of rows aligned in the [010] direction. By acquiring SPLEEM images along different spin directions the vector magnetization was mapped on the surface, both at room temperature and at a temperature well below the Verwey transition. At room temperature, domains were observed with their magnetization aligned along the two <111> bulk easy axes which are in the (110) surface plane. They presented 180$^\circ$, 71$^\circ$ and 109$^\circ$ Néel-type domain walls. Below the Verwey transition, the magnetization directions changed to regions where the magnetization was oriented along the in-plane [100] and [001] directions. Those observations can be interpreted as the presence of magnetized regions on the surface where the monoclinic $c$ axis is in-plane in the former, and regions where the $c$ is out-of-plane in an oblique direction in the latter. However, the magnetization was at all times within the surface plane, with no out-of-plane component detected.
format Preprint
id arxiv_https___arxiv_org_abs_2605_31252
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Magnetic domains reconfiguration on the Fe3O4(110) surface across the Verwey transition by Spin-Polarized Low-Energy Electron Microscopy
Gutiérrez-Cuesta, C.
Mandziak, A.
Prieto, J. E.
Nita, P.
Mascaraque, A.
Choudhry, U.
Turner, J.
Stibor, A.
de la Figuera, J.
Materials Science
We have studied the (110) surface of Fe$_3$O$_4$ single crystals by means of spin-polarized low-energy electron microscopy (SPLEEM). After preparation by sputtering and annealing a well defined reconstructed surface was achieved, composed of rows aligned in the [010] direction. By acquiring SPLEEM images along different spin directions the vector magnetization was mapped on the surface, both at room temperature and at a temperature well below the Verwey transition. At room temperature, domains were observed with their magnetization aligned along the two <111> bulk easy axes which are in the (110) surface plane. They presented 180$^\circ$, 71$^\circ$ and 109$^\circ$ Néel-type domain walls. Below the Verwey transition, the magnetization directions changed to regions where the magnetization was oriented along the in-plane [100] and [001] directions. Those observations can be interpreted as the presence of magnetized regions on the surface where the monoclinic $c$ axis is in-plane in the former, and regions where the $c$ is out-of-plane in an oblique direction in the latter. However, the magnetization was at all times within the surface plane, with no out-of-plane component detected.
title Magnetic domains reconfiguration on the Fe3O4(110) surface across the Verwey transition by Spin-Polarized Low-Energy Electron Microscopy
topic Materials Science
url https://arxiv.org/abs/2605.31252