Ferroelectric hysteresis in singly aligned graphene-hBN moiré superlattices

Fuente: arXiv
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Hauptverfasser: Tu, Bao Q., Ahmed, Tanweer, Avedissian, Garen, Lancaster, Suzanne, Sharma, Mayank, Watanabe, Kenji, Taniguchi, Takashi, Casanova, Fèlix, Gobbi, Marco, Hueso, Luis E.
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Veröffentlicht: 2026
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author Tu, Bao Q.
Ahmed, Tanweer
Avedissian, Garen
Lancaster, Suzanne
Sharma, Mayank
Watanabe, Kenji
Taniguchi, Takashi
Casanova, Fèlix
Gobbi, Marco
Hueso, Luis E.
author_facet Tu, Bao Q.
Ahmed, Tanweer
Avedissian, Garen
Lancaster, Suzanne
Sharma, Mayank
Watanabe, Kenji
Taniguchi, Takashi
Casanova, Fèlix
Gobbi, Marco
Hueso, Luis E.
contents Ferroelectric materials have the unique ability to maintain an electric polarization which can be reversed under an external applied electric field. This property makes them valuable for applications such as non-volatile random-access memories, transducers, actuators and electro optic modulators. Recently, emergent unconventional ferroelectricity has been demonstrated in moiré superlattices of bilayer graphene and hexagonal boron nitride (hBN) hosting non centrosymmetric stacking order. Whether this phenomenon is also present in noncentrosymmetric single layer graphene (SLG)-hBN moiré superlattices is still under debate. Here we demonstrate a ferroelectric response in an SLG-hBN moiré superlattice. Through Hall measurements, we pinpoint the origin of the hysteretic behavior to abnormal charge screening due to the moiré superlattice band and estimate the spontaneous polarization magnitude in the moiré superlattice structure. Temperature dependent measurements confirm that the hysteretic behavior persists from 2K up to room temperature, opening opportunities for high-mobility, ultrathin non-volatile devices
format Preprint
id arxiv_https___arxiv_org_abs_2606_02338
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Ferroelectric hysteresis in singly aligned graphene-hBN moiré superlattices
Tu, Bao Q.
Ahmed, Tanweer
Avedissian, Garen
Lancaster, Suzanne
Sharma, Mayank
Watanabe, Kenji
Taniguchi, Takashi
Casanova, Fèlix
Gobbi, Marco
Hueso, Luis E.
Mesoscale and Nanoscale Physics
Materials Science
Ferroelectric materials have the unique ability to maintain an electric polarization which can be reversed under an external applied electric field. This property makes them valuable for applications such as non-volatile random-access memories, transducers, actuators and electro optic modulators. Recently, emergent unconventional ferroelectricity has been demonstrated in moiré superlattices of bilayer graphene and hexagonal boron nitride (hBN) hosting non centrosymmetric stacking order. Whether this phenomenon is also present in noncentrosymmetric single layer graphene (SLG)-hBN moiré superlattices is still under debate. Here we demonstrate a ferroelectric response in an SLG-hBN moiré superlattice. Through Hall measurements, we pinpoint the origin of the hysteretic behavior to abnormal charge screening due to the moiré superlattice band and estimate the spontaneous polarization magnitude in the moiré superlattice structure. Temperature dependent measurements confirm that the hysteretic behavior persists from 2K up to room temperature, opening opportunities for high-mobility, ultrathin non-volatile devices
title Ferroelectric hysteresis in singly aligned graphene-hBN moiré superlattices
topic Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2606.02338