_version_ 1867171818707615744
author Rutgers van der Loeff, Michiel M
Cassar, Nicolas
Nicolaus, Marcel
Rabe, Benjamin
Stimac, Ingrid
author_facet Rutgers van der Loeff, Michiel M
Cassar, Nicolas
Nicolaus, Marcel
Rabe, Benjamin
Stimac, Ingrid
collection Datos científicos de ciencias marinas y ambientales
contents Air-sea gas exchange plays a key role in the cycling of greenhouse and other biogeochemically important gases. Although air-sea gas transfer is expected to change as a consequence of the rapid decline in summer Arctic sea ice cover, little is known about the effect of sea ice cover on gas exchange fluxes, especially in the marginal ice zone. During the Polarstern expedition ARK-XXVI/3 (TransArc, August/September 2011) to the central Arctic Ocean, we compared 222Rn/226Ra ratios in the upper 50 m of 14 ice-covered and 4 ice-free stations. At three of the ice-free stations, we find 222Rn-based gas transfer coefficients in good agreement with expectation based on published relationships between gas transfer and wind speed over open water when accounting for wind history from wind reanalysis data. We hypothesize that the low gas transfer rate at the fourth station results from reduced fetch due to the proximity of the ice edge, or lateral exchange across the front at the ice edge by restratification. No significant radon deficit could be observed at the ice-covered stations. At these stations, the average gas transfer velocity was less than 0.1 m/d (97.5% confidence), compared to 0.5-2.2 m/d expected for open water. Our results show that air-sea gas exchange in an ice-covered ocean is reduced by at least an order of magnitude compared to open water. In contrast to previous studies, we show that in partially ice-covered regions, gas exchange is lower than expected based on a linear scaling to percent ice cover.
format Dataset Open Access
id pangaea_https___doi_org_10_1594_PANGAEA_823179
institution PANGAEA
language en
publishDate 2014
publisher PANGAEA
record_format pangaea
spellingShingle Radon 222 and Radium 226 measured on water bottle samples during POLARSTERN cruise ARK-XXVI/3 (TransArc)
Rutgers van der Loeff, Michiel M
Cassar, Nicolas
Nicolaus, Marcel
Rabe, Benjamin
Stimac, Ingrid
Alpha-scintillation; Arctic Ocean; ARK-XXVI/3; AWI_MarGeoChem; Calculated; Date/Time of event; DEPTH, water; Elevation of event; Event label; Gamma-ray spectrometry; Laptev Sea; Latitude of event; Longitude of event; Marine Geochemistry @ AWI; MUWS; Polarstern; PS78/201-5; PS78/205-3; PS78/209-6; PS78/212-8; PS78/218-5; PS78/222-7; PS78/227-6; PS78/230-4; PS78/235-5; PS78/239-4; PS78/245-3; PS78/250-4; PS78/257-3; PS78/271-3; PS78/273-3; PS78/276-3; PS78/280-3; PS78/285-3; PS78 TransArc; Radium-226; Radium-226, normalized to salinity 35; Radium-226, standard deviation; Radon-222; Radon-222, standard deviation; Radon-222/Radium-226 activity ratio; Radon-222/Radium-226 activity ratio, standard deviation; Salinity; Water Multi Sampler
Air-sea gas exchange plays a key role in the cycling of greenhouse and other biogeochemically important gases. Although air-sea gas transfer is expected to change as a consequence of the rapid decline in summer Arctic sea ice cover, little is known about the effect of sea ice cover on gas exchange fluxes, especially in the marginal ice zone. During the Polarstern expedition ARK-XXVI/3 (TransArc, August/September 2011) to the central Arctic Ocean, we compared 222Rn/226Ra ratios in the upper 50 m of 14 ice-covered and 4 ice-free stations. At three of the ice-free stations, we find 222Rn-based gas transfer coefficients in good agreement with expectation based on published relationships between gas transfer and wind speed over open water when accounting for wind history from wind reanalysis data. We hypothesize that the low gas transfer rate at the fourth station results from reduced fetch due to the proximity of the ice edge, or lateral exchange across the front at the ice edge by restratification. No significant radon deficit could be observed at the ice-covered stations. At these stations, the average gas transfer velocity was less than 0.1 m/d (97.5% confidence), compared to 0.5-2.2 m/d expected for open water. Our results show that air-sea gas exchange in an ice-covered ocean is reduced by at least an order of magnitude compared to open water. In contrast to previous studies, we show that in partially ice-covered regions, gas exchange is lower than expected based on a linear scaling to percent ice cover.
title Radon 222 and Radium 226 measured on water bottle samples during POLARSTERN cruise ARK-XXVI/3 (TransArc)
topic Alpha-scintillation; Arctic Ocean; ARK-XXVI/3; AWI_MarGeoChem; Calculated; Date/Time of event; DEPTH, water; Elevation of event; Event label; Gamma-ray spectrometry; Laptev Sea; Latitude of event; Longitude of event; Marine Geochemistry @ AWI; MUWS; Polarstern; PS78/201-5; PS78/205-3; PS78/209-6; PS78/212-8; PS78/218-5; PS78/222-7; PS78/227-6; PS78/230-4; PS78/235-5; PS78/239-4; PS78/245-3; PS78/250-4; PS78/257-3; PS78/271-3; PS78/273-3; PS78/276-3; PS78/280-3; PS78/285-3; PS78 TransArc; Radium-226; Radium-226, normalized to salinity 35; Radium-226, standard deviation; Radon-222; Radon-222, standard deviation; Radon-222/Radium-226 activity ratio; Radon-222/Radium-226 activity ratio, standard deviation; Salinity; Water Multi Sampler
url https://doi.org/10.1594/PANGAEA.823179