Black Carbon measurements in Germany between 1994 and 2014, link to netCDF files

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Main Authors: Kutzner, Rebecca D, von Schneidemesser, Erika, Kuik, Friderike, Quedenau, Jörn, Weatherhead, Betsy, Schmale, Julia
Format: Dataset Open Access
Language:en
Published: PANGAEA 2017
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author Kutzner, Rebecca D
von Schneidemesser, Erika
Kuik, Friderike
Quedenau, Jörn
Weatherhead, Betsy
Schmale, Julia
author_facet Kutzner, Rebecca D
von Schneidemesser, Erika
Kuik, Friderike
Quedenau, Jörn
Weatherhead, Betsy
Schmale, Julia
collection Datos científicos de ciencias marinas y ambientales
contents Lately, black carbon (BC) has received significant attention due to its climate-warming properties and adverse health effects. Nevertheless, long-term observations in urban areas are scarce, most likely because BC monitoring is not required by environmental legislation. This, however, handicaps the evaluation of air quality models which can be used to assess the effectiveness of policy measures which aim at reducing BC concentrations. Here, we present a new dataset of atmospheric BC measurements from Germany constructed from over six million measurements at over 170 stations. Data covering the period between 1994 and 2014 were collected from twelve German federal states and the federal Environment Agency (UBA), quality checked and harmonized into a database with comprehensive metadata. The final data in original time resolution are available for download (link will follow). Though assembled in a consistent way, the dataset is characterized by differences in (a) measurement methodologies for determining evolved carbon and optical absorption, (b) covered time periods, and (c) temporal resolutions that ranged from half hourly to 6-daily measurements. Usage of this dataset thus requires a careful consideration of these differences. Our analysis focuses on 2009, the year with the largest data coverage obtained with one single methodology, as well as on the relative changes in long-term trends over ten years. Stations are grouped into the following categories: urban background, traffic, industrial, and rural. For 2009, we find that BC concentrations at traffic sites were at least twice as high as at urban background, industrial and rural sites. Weekly cycles are most prominent at traffic stations, however, the presence of differences in concentrations during the week and on weekends at other station types suggests that traffic plays an important role throughout the full network. Generally higher concentrations and weaker weekly cycles during the winter months point towards the influence of other sources such as domestic heating. Regarding the long-term trends, advanced statistical techniques allow us to account for instrumentation changes and to separate seasonal and long-term changes in our dataset. Analysis shows a downward trend in BC at nearly all locations and in all conditions, with a high level of confidence for the period of 2005-2014. In depth analysis indicates that background BC is decreasing slowly, while the occurrences of high concentrations are decreasing more rapidly. In summary, legislation - both in Europe and locally - to reduce particulate emissions and indirectly BC appear to be working, based on this analysis. Human health and climate impacts are likely to be diminished because of the improvements in air quality.
format Dataset Open Access
id pangaea_https___doi_org_10_1594_PANGAEA_881173
institution PANGAEA
language en
publishDate 2017
publisher PANGAEA
record_format pangaea
spellingShingle Black Carbon measurements in Germany between 1994 and 2014, link to netCDF files
Kutzner, Rebecca D
von Schneidemesser, Erika
Kuik, Friderike
Quedenau, Jörn
Weatherhead, Betsy
Schmale, Julia
Germany; MULT; Multiple investigations
Lately, black carbon (BC) has received significant attention due to its climate-warming properties and adverse health effects. Nevertheless, long-term observations in urban areas are scarce, most likely because BC monitoring is not required by environmental legislation. This, however, handicaps the evaluation of air quality models which can be used to assess the effectiveness of policy measures which aim at reducing BC concentrations. Here, we present a new dataset of atmospheric BC measurements from Germany constructed from over six million measurements at over 170 stations. Data covering the period between 1994 and 2014 were collected from twelve German federal states and the federal Environment Agency (UBA), quality checked and harmonized into a database with comprehensive metadata. The final data in original time resolution are available for download (link will follow). Though assembled in a consistent way, the dataset is characterized by differences in (a) measurement methodologies for determining evolved carbon and optical absorption, (b) covered time periods, and (c) temporal resolutions that ranged from half hourly to 6-daily measurements. Usage of this dataset thus requires a careful consideration of these differences. Our analysis focuses on 2009, the year with the largest data coverage obtained with one single methodology, as well as on the relative changes in long-term trends over ten years. Stations are grouped into the following categories: urban background, traffic, industrial, and rural. For 2009, we find that BC concentrations at traffic sites were at least twice as high as at urban background, industrial and rural sites. Weekly cycles are most prominent at traffic stations, however, the presence of differences in concentrations during the week and on weekends at other station types suggests that traffic plays an important role throughout the full network. Generally higher concentrations and weaker weekly cycles during the winter months point towards the influence of other sources such as domestic heating. Regarding the long-term trends, advanced statistical techniques allow us to account for instrumentation changes and to separate seasonal and long-term changes in our dataset. Analysis shows a downward trend in BC at nearly all locations and in all conditions, with a high level of confidence for the period of 2005-2014. In depth analysis indicates that background BC is decreasing slowly, while the occurrences of high concentrations are decreasing more rapidly. In summary, legislation - both in Europe and locally - to reduce particulate emissions and indirectly BC appear to be working, based on this analysis. Human health and climate impacts are likely to be diminished because of the improvements in air quality.
title Black Carbon measurements in Germany between 1994 and 2014, link to netCDF files
topic Germany; MULT; Multiple investigations
url https://doi.org/10.1594/PANGAEA.881173