Evidence for millennial-scale interactions between Hg cycling and hydroclimate from Lake Bosumtwi, Ghana

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Main Authors: Paine, Alice R, Frieling, Joost, Shanahan, Timothy M, Mather, Tamsin A, McKay, Nicholas, Robinson, Stuart A, Pyle, David M, Fendley, Isabel M, Kiely, R, Gosling, William D
Format: Dataset Open Access
Language:en
Published: PANGAEA 2025
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author Paine, Alice R
Frieling, Joost
Shanahan, Timothy M
Mather, Tamsin A
McKay, Nicholas
Robinson, Stuart A
Pyle, David M
Fendley, Isabel M
Kiely, R
Gosling, William D
author_facet Paine, Alice R
Frieling, Joost
Shanahan, Timothy M
Mather, Tamsin A
McKay, Nicholas
Robinson, Stuart A
Pyle, David M
Fendley, Isabel M
Kiely, R
Gosling, William D
collection Datos científicos de ciencias marinas y ambientales
contents The datasets include measurements of mercury, total organic, and inorganic carbon in sediment samples from core BOS04-5B, extracted from Lake Bosumtwi in 2004 as part of the ICDP Lake Bosumtwi Drilling Project. Lake Bosumtwi is the only natural lake in Ghana, western Africa (6°300 N, 1°250 W), and occupies a meteorite impact crater dated to 1.08 ± 0.04 Ma: one of the youngest and best-preserved impact craters on Earth. Focusing on the uppermost ∼ 47 m of the BOS04-5B sediment record, this data was generated to assesses whether major shifts in local hydroclimate produced measurable changes in how Hg has been transported to, and buried within, this system since ∼ 96 ka. Total Hg (HgT) in the bulk sediments of the core was measured using an RA-915 portable mercury analyser with a PYRO-915+ pyrolyser, Lumex, at the University of Oxford (UK). For this study, we analysed 165 samples spanning the composite depth interval 47.7 to 0 m, with an average temporal resolution of ∼ 0.6 ka between each sample (range: 0.01 to 5.85 kyr). Quantitative values for total organic carbon (TOC) and total inorganic carbon (TIC) content were measured on the same powdered sample material also analysed for Hg, using a Stroehlein Coulomat 702 at the University of Oxford (UK). Analytical reproducibility for this instrument was ≤ 0.2% based on repeat measurements, with a detection limit of ca. 0.1 %-0.2 %.
format Dataset Open Access
id pangaea_https___doi_org_10_1594_PANGAEA_981521
institution PANGAEA
language en
publishDate 2025
publisher PANGAEA
record_format pangaea
spellingShingle Evidence for millennial-scale interactions between Hg cycling and hydroclimate from Lake Bosumtwi, Ghana
Paine, Alice R
Frieling, Joost
Shanahan, Timothy M
Mather, Tamsin A
McKay, Nicholas
Robinson, Stuart A
Pyle, David M
Fendley, Isabel M
Kiely, R
Gosling, William D
Accumulation rate, mercury; AGE; biogeochemical cycles; Calculated; Carbon, inorganic, total; Carbon, organic, total; Core; CORE; Core section label; Coulomat, STRÖHLEIN, 702; Density, dry bulk; DEPTH, sediment/rock; GLAD6_BOS04_5B; Lake Bosumtwi, Ghana; lake sediment proxies; Mercury; Mercury analyzer, Lumex Instruments, RA-915M; coupled with PYRO-915+ thermal decomposition attachment; organic carbon content; XRF
The datasets include measurements of mercury, total organic, and inorganic carbon in sediment samples from core BOS04-5B, extracted from Lake Bosumtwi in 2004 as part of the ICDP Lake Bosumtwi Drilling Project. Lake Bosumtwi is the only natural lake in Ghana, western Africa (6°300 N, 1°250 W), and occupies a meteorite impact crater dated to 1.08 ± 0.04 Ma: one of the youngest and best-preserved impact craters on Earth. Focusing on the uppermost ∼ 47 m of the BOS04-5B sediment record, this data was generated to assesses whether major shifts in local hydroclimate produced measurable changes in how Hg has been transported to, and buried within, this system since ∼ 96 ka. Total Hg (HgT) in the bulk sediments of the core was measured using an RA-915 portable mercury analyser with a PYRO-915+ pyrolyser, Lumex, at the University of Oxford (UK). For this study, we analysed 165 samples spanning the composite depth interval 47.7 to 0 m, with an average temporal resolution of ∼ 0.6 ka between each sample (range: 0.01 to 5.85 kyr). Quantitative values for total organic carbon (TOC) and total inorganic carbon (TIC) content were measured on the same powdered sample material also analysed for Hg, using a Stroehlein Coulomat 702 at the University of Oxford (UK). Analytical reproducibility for this instrument was ≤ 0.2% based on repeat measurements, with a detection limit of ca. 0.1 %-0.2 %.
title Evidence for millennial-scale interactions between Hg cycling and hydroclimate from Lake Bosumtwi, Ghana
topic Accumulation rate, mercury; AGE; biogeochemical cycles; Calculated; Carbon, inorganic, total; Carbon, organic, total; Core; CORE; Core section label; Coulomat, STRÖHLEIN, 702; Density, dry bulk; DEPTH, sediment/rock; GLAD6_BOS04_5B; Lake Bosumtwi, Ghana; lake sediment proxies; Mercury; Mercury analyzer, Lumex Instruments, RA-915M; coupled with PYRO-915+ thermal decomposition attachment; organic carbon content; XRF
url https://doi.org/10.1594/PANGAEA.981521