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Main Authors: Hu, Le, Liu, Qing, Wang, Yuxin, Wang, Chunxiao, Fan, Yinuo, Liu, Shuying, Shi, Yujiao, Jin, Kang, Tan, Wei-Qiang, Pan, Panpan, Chen, Jingdi
Format: Artículo científico
Language:en
Published: ACS applied materials & interfaces 2025
Subjects:
Online Access:https://pubmed.ncbi.nlm.nih.gov/40025822/
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author Hu, Le
Liu, Qing
Wang, Yuxin
Wang, Chunxiao
Fan, Yinuo
Liu, Shuying
Shi, Yujiao
Jin, Kang
Tan, Wei-Qiang
Pan, Panpan
Chen, Jingdi
author_facet Hu, Le
Liu, Qing
Wang, Yuxin
Wang, Chunxiao
Fan, Yinuo
Liu, Shuying
Shi, Yujiao
Jin, Kang
Tan, Wei-Qiang
Pan, Panpan
Chen, Jingdi
Hu, Le
Liu, Qing
Wang, Yuxin
Wang, Chunxiao
Fan, Yinuo
Liu, Shuying
Shi, Yujiao
Jin, Kang
Tan, Wei-Qiang
Pan, Panpan
Chen, Jingdi
collection PubMed - marine biology
contents A Semi-Interpenetrating Network Hydrogel with Excellent Photothermal Antibacterial and ROS Scavenging Activities for MRSA-Infected Wounds. Hu, Le Liu, Qing Wang, Yuxin Wang, Chunxiao Fan, Yinuo Liu, Shuying Shi, Yujiao Jin, Kang Tan, Wei-Qiang Pan, Panpan Chen, Jingdi Hydrogels Methicillin-Resistant Staphylococcus aureus Animals Anti-Bacterial Agents Rats Rats, Sprague-Dawley Reactive Oxygen Species Wound Healing Staphylococcal Infections Dopamine Wound Infection Polysaccharides, Bacterial Free Radical Scavengers Nanoparticles Male Microbial Sensitivity Tests Ferrocyanides The prolonged infection of bacteria at the wound site may lead to serious physical problems. Herein, a multifunctional macroporous hydrogel with superior photothermal antibacterial and ROS scavenging activity (denoted as M-XG gel) was designed for the treatment of MRSA-infected wounds. The M-XG gels are composed of embedding Prussian blue nanoparticles (PBNPs) as photothermal converters and chelating ferric ions with xanthan gum (XG) and dopamine (DA) to form a semipermeable network. The introduction of DA occupies the cross-link sites of ferric ions, further increasing the pore size (200-500 μm open macropores) and endowing the hydrogel with ideal adhesion. The increase of cross-link sites in PBNPs formed a promising equilibrium M-XG gel with identical macroporous structures and toughened mechanical performance. The metal ligands between ferric ions and catechols, as well as the unique photothermal response of PBNPs, endow the hydrogels with a fast and stable near-infrared (NIR) photothermal conversion efficiency (48%). In the MRSA-infected SD rat trauma model, wounds treated with the M-XG gel group had completely closed after 14 days, effectively controlling wound bacterial infection and accelerating angiogenesis and collagen deposition, synergistically promoting infected wound healing. Therefore, the photothermal hydrogel with a semi-interpenetrating network demonstrates its great potential for infected wound tissue engineering.
format Artículo científico
id pubmed_40025822
institution PubMed
language en
publishDate 2025
publisher ACS applied materials & interfaces
record_format pubmed
spellingShingle A Semi-Interpenetrating Network Hydrogel with Excellent Photothermal Antibacterial and ROS Scavenging Activities for MRSA-Infected Wounds.
Hu, Le
Liu, Qing
Wang, Yuxin
Wang, Chunxiao
Fan, Yinuo
Liu, Shuying
Shi, Yujiao
Jin, Kang
Tan, Wei-Qiang
Pan, Panpan
Chen, Jingdi
Hydrogels
Methicillin-Resistant Staphylococcus aureus
Animals
Anti-Bacterial Agents
Rats
Rats, Sprague-Dawley
Reactive Oxygen Species
Wound Healing
Staphylococcal Infections
Dopamine
Wound Infection
Polysaccharides, Bacterial
Free Radical Scavengers
Nanoparticles
Male
Microbial Sensitivity Tests
Ferrocyanides
A Semi-Interpenetrating Network Hydrogel with Excellent Photothermal Antibacterial and ROS Scavenging Activities for MRSA-Infected Wounds. Hu, Le Liu, Qing Wang, Yuxin Wang, Chunxiao Fan, Yinuo Liu, Shuying Shi, Yujiao Jin, Kang Tan, Wei-Qiang Pan, Panpan Chen, Jingdi Hydrogels Methicillin-Resistant Staphylococcus aureus Animals Anti-Bacterial Agents Rats Rats, Sprague-Dawley Reactive Oxygen Species Wound Healing Staphylococcal Infections Dopamine Wound Infection Polysaccharides, Bacterial Free Radical Scavengers Nanoparticles Male Microbial Sensitivity Tests Ferrocyanides The prolonged infection of bacteria at the wound site may lead to serious physical problems. Herein, a multifunctional macroporous hydrogel with superior photothermal antibacterial and ROS scavenging activity (denoted as M-XG gel) was designed for the treatment of MRSA-infected wounds. The M-XG gels are composed of embedding Prussian blue nanoparticles (PBNPs) as photothermal converters and chelating ferric ions with xanthan gum (XG) and dopamine (DA) to form a semipermeable network. The introduction of DA occupies the cross-link sites of ferric ions, further increasing the pore size (200-500 μm open macropores) and endowing the hydrogel with ideal adhesion. The increase of cross-link sites in PBNPs formed a promising equilibrium M-XG gel with identical macroporous structures and toughened mechanical performance. The metal ligands between ferric ions and catechols, as well as the unique photothermal response of PBNPs, endow the hydrogels with a fast and stable near-infrared (NIR) photothermal conversion efficiency (48%). In the MRSA-infected SD rat trauma model, wounds treated with the M-XG gel group had completely closed after 14 days, effectively controlling wound bacterial infection and accelerating angiogenesis and collagen deposition, synergistically promoting infected wound healing. Therefore, the photothermal hydrogel with a semi-interpenetrating network demonstrates its great potential for infected wound tissue engineering.
title A Semi-Interpenetrating Network Hydrogel with Excellent Photothermal Antibacterial and ROS Scavenging Activities for MRSA-Infected Wounds.
topic Hydrogels
Methicillin-Resistant Staphylococcus aureus
Animals
Anti-Bacterial Agents
Rats
Rats, Sprague-Dawley
Reactive Oxygen Species
Wound Healing
Staphylococcal Infections
Dopamine
Wound Infection
Polysaccharides, Bacterial
Free Radical Scavengers
Nanoparticles
Male
Microbial Sensitivity Tests
Ferrocyanides
url https://pubmed.ncbi.nlm.nih.gov/40025822/