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Main Authors: Yu, Chunlin, Wang, Zhanhua, Wang, Wenjie, Li, Rongfeng, Xing, Ronge, Liu, Song, Li, Pengcheng, Yu, Huahua
Format: Artículo científico
Language:en
Published: Archives of toxicology 2026
Subjects:
Online Access:https://pubmed.ncbi.nlm.nih.gov/41162771/
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author Yu, Chunlin
Wang, Zhanhua
Wang, Wenjie
Li, Rongfeng
Xing, Ronge
Liu, Song
Li, Pengcheng
Yu, Huahua
author_facet Yu, Chunlin
Wang, Zhanhua
Wang, Wenjie
Li, Rongfeng
Xing, Ronge
Liu, Song
Li, Pengcheng
Yu, Huahua
Yu, Chunlin
Wang, Zhanhua
Wang, Wenjie
Li, Rongfeng
Xing, Ronge
Liu, Song
Li, Pengcheng
Yu, Huahua
collection PubMed - marine biology
contents Targeting marine jellyfish toxins: development of metalloproteinase inhibitors through a specific method for protease substrate identification. Yu, Chunlin Wang, Zhanhua Wang, Wenjie Li, Rongfeng Xing, Ronge Liu, Song Li, Pengcheng Yu, Huahua Animals Mice Cnidarian Venoms Metalloproteases RAW 264.7 Cells Scyphozoa Peptide Library Peptides Marine Toxins Protease Inhibitors Substrate Specificity The venom of hazardous jellyfish contains harmful substances to human health, such as metalloproteinases, which are challenging to purify. Therefore, identifying substrate sequences using crude venom is crucial for the development of peptide inhibitors. This study utilized a designed peptide library and an abundance-based hydrolysis product analysis approach to identify the substrate sequences of toxin metalloproteinases from Nemopilema nomurai nematocyst venom (NnNV) and further modified these sequences into peptide inhibitors. Specifically, a peptide library comprising 41 potential substrate sequences was constructed and incubated with NnNV. 12 substrate sequences and 14 cleavage sites were identified from the hydrolysis products. In the design of peptide inhibitors, thiol (-SH) and phosphate groups (-POH) were used as zinc-binding groups, and sixty derived peptides were obtained. 15 peptide inhibitors were selected for their efficacy in inhibiting toxin metalloproteinase activity, with CPRGQPIIQDV demonstrating the most potent effect. CPRGQPIIQDV mainly presented β-sheet and random coil structures, and significantly reduced the cytotoxicity and pro-inflammatory effects of NnNV on RAW264.7 cells. This study established a method for identifying metalloproteinase substrate sequences using crude jellyfish venom and provided an initial design and screening of peptide inhibitors, offering new insights into the management of jellyfish stings.
format Artículo científico
id pubmed_41162771
institution PubMed
language en
publishDate 2026
publisher Archives of toxicology
record_format pubmed
spellingShingle Targeting marine jellyfish toxins: development of metalloproteinase inhibitors through a specific method for protease substrate identification.
Yu, Chunlin
Wang, Zhanhua
Wang, Wenjie
Li, Rongfeng
Xing, Ronge
Liu, Song
Li, Pengcheng
Yu, Huahua
Animals
Mice
Cnidarian Venoms
Metalloproteases
RAW 264.7 Cells
Scyphozoa
Peptide Library
Peptides
Marine Toxins
Protease Inhibitors
Substrate Specificity
Targeting marine jellyfish toxins: development of metalloproteinase inhibitors through a specific method for protease substrate identification. Yu, Chunlin Wang, Zhanhua Wang, Wenjie Li, Rongfeng Xing, Ronge Liu, Song Li, Pengcheng Yu, Huahua Animals Mice Cnidarian Venoms Metalloproteases RAW 264.7 Cells Scyphozoa Peptide Library Peptides Marine Toxins Protease Inhibitors Substrate Specificity The venom of hazardous jellyfish contains harmful substances to human health, such as metalloproteinases, which are challenging to purify. Therefore, identifying substrate sequences using crude venom is crucial for the development of peptide inhibitors. This study utilized a designed peptide library and an abundance-based hydrolysis product analysis approach to identify the substrate sequences of toxin metalloproteinases from Nemopilema nomurai nematocyst venom (NnNV) and further modified these sequences into peptide inhibitors. Specifically, a peptide library comprising 41 potential substrate sequences was constructed and incubated with NnNV. 12 substrate sequences and 14 cleavage sites were identified from the hydrolysis products. In the design of peptide inhibitors, thiol (-SH) and phosphate groups (-POH) were used as zinc-binding groups, and sixty derived peptides were obtained. 15 peptide inhibitors were selected for their efficacy in inhibiting toxin metalloproteinase activity, with CPRGQPIIQDV demonstrating the most potent effect. CPRGQPIIQDV mainly presented β-sheet and random coil structures, and significantly reduced the cytotoxicity and pro-inflammatory effects of NnNV on RAW264.7 cells. This study established a method for identifying metalloproteinase substrate sequences using crude jellyfish venom and provided an initial design and screening of peptide inhibitors, offering new insights into the management of jellyfish stings.
title Targeting marine jellyfish toxins: development of metalloproteinase inhibitors through a specific method for protease substrate identification.
topic Animals
Mice
Cnidarian Venoms
Metalloproteases
RAW 264.7 Cells
Scyphozoa
Peptide Library
Peptides
Marine Toxins
Protease Inhibitors
Substrate Specificity
url https://pubmed.ncbi.nlm.nih.gov/41162771/