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Main Authors: Wang, Ning, Westermann, Linda M, Li, Mingyu, Li, Chun-Yang, Murphy, Andrew R J, Gu, Zengtian, Silvano, Eleonora, Blindauer, Claudia A, Lidbury, Ian D E A, Zhang, Yu-Zhong, Scanlan, David J, Chen, Yin
Format: Artículo científico
Language:en
Published: Proceedings of the National Academy of Sciences of the United States of America 2025
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Online Access:https://pubmed.ncbi.nlm.nih.gov/41364767/
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author Wang, Ning
Westermann, Linda M
Li, Mingyu
Li, Chun-Yang
Murphy, Andrew R J
Gu, Zengtian
Silvano, Eleonora
Blindauer, Claudia A
Lidbury, Ian D E A
Zhang, Yu-Zhong
Scanlan, David J
Chen, Yin
author_facet Wang, Ning
Westermann, Linda M
Li, Mingyu
Li, Chun-Yang
Murphy, Andrew R J
Gu, Zengtian
Silvano, Eleonora
Blindauer, Claudia A
Lidbury, Ian D E A
Zhang, Yu-Zhong
Scanlan, David J
Chen, Yin
Wang, Ning
Westermann, Linda M
Li, Mingyu
Li, Chun-Yang
Murphy, Andrew R J
Gu, Zengtian
Silvano, Eleonora
Blindauer, Claudia A
Lidbury, Ian D E A
Zhang, Yu-Zhong
Scanlan, David J
Chen, Yin
collection PubMed - marine biology
contents Structural basis and evolutionary pathways of glycerol-1-phosphate transport in marine bacteria. Wang, Ning Westermann, Linda M Li, Mingyu Li, Chun-Yang Murphy, Andrew R J Gu, Zengtian Silvano, Eleonora Blindauer, Claudia A Lidbury, Ian D E A Zhang, Yu-Zhong Scanlan, David J Chen, Yin Phylogeny Glycerophosphates Evolution, Molecular Bacterial Proteins Biological Transport Bacteria Aquatic Organisms Seawater Membrane Transport Proteins All cells use lipid membranes to maintain cellular integrity and function, though Archaea utilize lipids composed of glycerol-1-phosphate (G1P), while Bacteria and Eukaryotes use glycerol-3-phosphate (G3P). Given that Archaea contribute significantly to global marine biomass, accounting for 0.3 gigatonnes (Gt) of carbon in the oceans, we aimed to uncover how archaeal G1P is recycled by marine microorganisms. Through a multidisciplinary approach combining microbiology, biochemistry, and structural biology, we identified a G1P transporter in marine bacteria, which we named GpxB. Phylogenetic analysis revealed that GpxB belongs to the organic phosphonate transporter (PhnT) family and is widely distributed in the marine microbiome, found in approximately 5 to 10% of microbial cells in surface marine waters. Strikingly, we also identified a second G1P transporter, UgpB, that is known to transport G3P and belongs to the carbohydrate uptake transporter-1 (CUT1) family, in the model bacterium sp. MED193. To explore the evolutionary pathways that led to the formation of G1P binding sites in both the PhnT and CUT1 families, we determined the structures of GpxB and UgpB bound to G1P and G3P. Using structure-guided mutagenesis and a comparative analysis of the binding pockets within the PhnT and CUT1 families, we traced their evolutionary trajectories, highlighting the distinct strategies through which G1P-binding sites developed in these two protein families.
format Artículo científico
id pubmed_41364767
institution PubMed
language en
publishDate 2025
publisher Proceedings of the National Academy of Sciences of the United States of America
record_format pubmed
spellingShingle Structural basis and evolutionary pathways of glycerol-1-phosphate transport in marine bacteria.
Wang, Ning
Westermann, Linda M
Li, Mingyu
Li, Chun-Yang
Murphy, Andrew R J
Gu, Zengtian
Silvano, Eleonora
Blindauer, Claudia A
Lidbury, Ian D E A
Zhang, Yu-Zhong
Scanlan, David J
Chen, Yin
Phylogeny
Glycerophosphates
Evolution, Molecular
Bacterial Proteins
Biological Transport
Bacteria
Aquatic Organisms
Seawater
Membrane Transport Proteins
Structural basis and evolutionary pathways of glycerol-1-phosphate transport in marine bacteria. Wang, Ning Westermann, Linda M Li, Mingyu Li, Chun-Yang Murphy, Andrew R J Gu, Zengtian Silvano, Eleonora Blindauer, Claudia A Lidbury, Ian D E A Zhang, Yu-Zhong Scanlan, David J Chen, Yin Phylogeny Glycerophosphates Evolution, Molecular Bacterial Proteins Biological Transport Bacteria Aquatic Organisms Seawater Membrane Transport Proteins All cells use lipid membranes to maintain cellular integrity and function, though Archaea utilize lipids composed of glycerol-1-phosphate (G1P), while Bacteria and Eukaryotes use glycerol-3-phosphate (G3P). Given that Archaea contribute significantly to global marine biomass, accounting for 0.3 gigatonnes (Gt) of carbon in the oceans, we aimed to uncover how archaeal G1P is recycled by marine microorganisms. Through a multidisciplinary approach combining microbiology, biochemistry, and structural biology, we identified a G1P transporter in marine bacteria, which we named GpxB. Phylogenetic analysis revealed that GpxB belongs to the organic phosphonate transporter (PhnT) family and is widely distributed in the marine microbiome, found in approximately 5 to 10% of microbial cells in surface marine waters. Strikingly, we also identified a second G1P transporter, UgpB, that is known to transport G3P and belongs to the carbohydrate uptake transporter-1 (CUT1) family, in the model bacterium sp. MED193. To explore the evolutionary pathways that led to the formation of G1P binding sites in both the PhnT and CUT1 families, we determined the structures of GpxB and UgpB bound to G1P and G3P. Using structure-guided mutagenesis and a comparative analysis of the binding pockets within the PhnT and CUT1 families, we traced their evolutionary trajectories, highlighting the distinct strategies through which G1P-binding sites developed in these two protein families.
title Structural basis and evolutionary pathways of glycerol-1-phosphate transport in marine bacteria.
topic Phylogeny
Glycerophosphates
Evolution, Molecular
Bacterial Proteins
Biological Transport
Bacteria
Aquatic Organisms
Seawater
Membrane Transport Proteins
url https://pubmed.ncbi.nlm.nih.gov/41364767/