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Autores principales: Carvalho, João P F, Teixeira, Maria C, Luís, Jorge L, Tavares, Bernardo L, Oliveira, Helena, Oliveira, José M, Silvestre, Armando J D, Vilela, Carla, Freire, Carmen S R
Formato: Artículo científico
Lenguaje:en
Publicado: International journal of biological macromolecules 2026
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Acceso en línea:https://pubmed.ncbi.nlm.nih.gov/41905690/
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author Carvalho, João P F
Teixeira, Maria C
Luís, Jorge L
Tavares, Bernardo L
Oliveira, Helena
Oliveira, José M
Silvestre, Armando J D
Vilela, Carla
Freire, Carmen S R
author_facet Carvalho, João P F
Teixeira, Maria C
Luís, Jorge L
Tavares, Bernardo L
Oliveira, Helena
Oliveira, José M
Silvestre, Armando J D
Vilela, Carla
Freire, Carmen S R
Carvalho, João P F
Teixeira, Maria C
Luís, Jorge L
Tavares, Bernardo L
Oliveira, Helena
Oliveira, José M
Silvestre, Armando J D
Vilela, Carla
Freire, Carmen S R
collection PubMed - marine biology
contents Conductive and antioxidant biopolymeric hydrogel-based bioinks with nanohybrids of protein amyloid nanofibrils‑gold nanoparticles for cardiac 3D bioprinting. Carvalho, João P F Teixeira, Maria C Luís, Jorge L Tavares, Bernardo L Oliveira, Helena Oliveira, José M Silvestre, Armando J D Vilela, Carla Freire, Carmen S R Antioxidants Hydrogels Ink Bioprinting Metal Nanoparticles Amyloid Gold Heart Myocytes, Cardiac Animals Rats Cell Line Tissue Engineering 3D bioprinting is a versatile technique that combines living cells and biomaterials to fabricate in vitro 3D living structures that resemble native tissues. These 3D platforms, with a higher complexity than traditional 2D cell cultures, emerge as new alternatives for biomedical research and tissue engineering. In this work, high performance conductive bioinks were developed by the combination of a hydrogel matrix of gellan gum (1.5 wt%) and carboxymethyl cellulose (1.0 wt%) with hybrid nanostructures composed of lysozyme amyloid nanofibrils and gold nanoparticles (LNF:AuNPs). The ink formulations show proper rheological properties, with a shear-thinning behavior and good elastic modulus (G') recovery rate (>85%), notorious printability, and enhanced conductivity (~3.0 mS cm) granted by the presence of LNF:AuNPs, viz. Ink_LNF:AuNPs_5% and Ink_LNF:AuNPs_15%. Moreover, the resulting hydrogels mimic the stiffness of myocardium (70%), and the incorporation of LNF:AuNPs reduces their degradation rate (from above 30% to 13.8 ± 2.4%) and improves their antioxidant activity (from 22.0 ± 0.8% to 75.1 ± 0.3%). The successful 3D bioprinting of bioinks laden with cardiomyocytes (H9c2 cells) originates complex structures that maintain high cell viability (90%) for 7 days, confirming their biocompatibility and potential for the 3D bioprinting of living structures that could be used as cardiac tissue platforms for different purposes.
format Artículo científico
id pubmed_41905690
institution PubMed
language en
publishDate 2026
publisher International journal of biological macromolecules
record_format pubmed
spellingShingle Conductive and antioxidant biopolymeric hydrogel-based bioinks with nanohybrids of protein amyloid nanofibrils‑gold nanoparticles for cardiac 3D bioprinting.
Carvalho, João P F
Teixeira, Maria C
Luís, Jorge L
Tavares, Bernardo L
Oliveira, Helena
Oliveira, José M
Silvestre, Armando J D
Vilela, Carla
Freire, Carmen S R
Antioxidants
Hydrogels
Ink
Bioprinting
Metal Nanoparticles
Amyloid
Gold
Heart
Myocytes, Cardiac
Animals
Rats
Cell Line
Tissue Engineering
Conductive and antioxidant biopolymeric hydrogel-based bioinks with nanohybrids of protein amyloid nanofibrils‑gold nanoparticles for cardiac 3D bioprinting. Carvalho, João P F Teixeira, Maria C Luís, Jorge L Tavares, Bernardo L Oliveira, Helena Oliveira, José M Silvestre, Armando J D Vilela, Carla Freire, Carmen S R Antioxidants Hydrogels Ink Bioprinting Metal Nanoparticles Amyloid Gold Heart Myocytes, Cardiac Animals Rats Cell Line Tissue Engineering 3D bioprinting is a versatile technique that combines living cells and biomaterials to fabricate in vitro 3D living structures that resemble native tissues. These 3D platforms, with a higher complexity than traditional 2D cell cultures, emerge as new alternatives for biomedical research and tissue engineering. In this work, high performance conductive bioinks were developed by the combination of a hydrogel matrix of gellan gum (1.5 wt%) and carboxymethyl cellulose (1.0 wt%) with hybrid nanostructures composed of lysozyme amyloid nanofibrils and gold nanoparticles (LNF:AuNPs). The ink formulations show proper rheological properties, with a shear-thinning behavior and good elastic modulus (G') recovery rate (>85%), notorious printability, and enhanced conductivity (~3.0 mS cm) granted by the presence of LNF:AuNPs, viz. Ink_LNF:AuNPs_5% and Ink_LNF:AuNPs_15%. Moreover, the resulting hydrogels mimic the stiffness of myocardium (70%), and the incorporation of LNF:AuNPs reduces their degradation rate (from above 30% to 13.8 ± 2.4%) and improves their antioxidant activity (from 22.0 ± 0.8% to 75.1 ± 0.3%). The successful 3D bioprinting of bioinks laden with cardiomyocytes (H9c2 cells) originates complex structures that maintain high cell viability (90%) for 7 days, confirming their biocompatibility and potential for the 3D bioprinting of living structures that could be used as cardiac tissue platforms for different purposes.
title Conductive and antioxidant biopolymeric hydrogel-based bioinks with nanohybrids of protein amyloid nanofibrils‑gold nanoparticles for cardiac 3D bioprinting.
topic Antioxidants
Hydrogels
Ink
Bioprinting
Metal Nanoparticles
Amyloid
Gold
Heart
Myocytes, Cardiac
Animals
Rats
Cell Line
Tissue Engineering
url https://pubmed.ncbi.nlm.nih.gov/41905690/