Formal synthesis of (±)-γ−Lycorane

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1. Verfasser: Yazmín M. Osornio
Format: Artículo científico
Sprache:en
Veröffentlicht: Sociedad Química de México 2004
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author Yazmín M. Osornio
author_facet Yazmín M. Osornio
contents Formal synthesis of (±)-γ−Lycorane Yazmín M. Osornio Luis D. Miranda Multidisciplinaria (Ciencias Naturales y Exactas) &#947 lycorane alkaloids xanthates radical cyclization A formal synthesis of (±)-γ-lycorane 4 based on the generationof the tetracyclic ketone 5 is disclosed. The general strategy ofthe synthesis of 5 rests on the rapid construction of the highly functionalizedintermediates 6 or 20 by a xanthate-based radical additioncyclization-oxidation cascade process, followed by either, a Friedel-Crafts type cyclization of 17 or a Dieckmann cyclization-decarboalkoxylationsequence on 21. 2004 artículo científico 1870-249X https://www.redalyc.org/articulo.oa?id=47548415 en http://www.redalyc.org/revista.oa?id=475 Journal of the Mexican Chemical Society application/pdf Sociedad Química de México Journal of the Mexican Chemical Society (México) Num.4 Vol.48
format Artículo científico
id redalyc_47548415
institution Redalyc
language en
publishDate 2004
publisher Sociedad Química de México
spellingShingle Formal synthesis of (±)-γ−Lycorane
Yazmín M. Osornio
Multidisciplinaria (Ciencias Naturales y Exactas)
&#947
lycorane
alkaloids
xanthates
radical cyclization
Formal synthesis of (±)-γ−Lycorane Yazmín M. Osornio Luis D. Miranda Multidisciplinaria (Ciencias Naturales y Exactas) &#947 lycorane alkaloids xanthates radical cyclization A formal synthesis of (±)-γ-lycorane 4 based on the generationof the tetracyclic ketone 5 is disclosed. The general strategy ofthe synthesis of 5 rests on the rapid construction of the highly functionalizedintermediates 6 or 20 by a xanthate-based radical additioncyclization-oxidation cascade process, followed by either, a Friedel-Crafts type cyclization of 17 or a Dieckmann cyclization-decarboalkoxylationsequence on 21. 2004 artículo científico 1870-249X https://www.redalyc.org/articulo.oa?id=47548415 en http://www.redalyc.org/revista.oa?id=475 Journal of the Mexican Chemical Society application/pdf Sociedad Química de México Journal of the Mexican Chemical Society (México) Num.4 Vol.48
title Formal synthesis of (±)-γ−Lycorane
topic Multidisciplinaria (Ciencias Naturales y Exactas)
&#947
lycorane
alkaloids
xanthates
radical cyclization
url https://www.redalyc.org/articulo.oa?id=47548415