EFFECT OF THE ADDITION OF PHOSPHOTUNGSTIC ACID ON THE THERMAL STABILITY OF ZIRCONIUM OXIDE

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Autore principale: JUAN MANUEL HERNÁNDEZ-ENRÍQUEZ
Natura: Artículo científico
Lingua:en
Pubblicazione: Universidad Nacional de Colombia 2014
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author JUAN MANUEL HERNÁNDEZ-ENRÍQUEZ
author_facet JUAN MANUEL HERNÁNDEZ-ENRÍQUEZ
contents EFFECT OF THE ADDITION OF PHOSPHOTUNGSTIC ACID ON THE THERMAL STABILITY OF ZIRCONIUM OXIDE JUAN MANUEL HERNÁNDEZ-ENRÍQUEZ RICARDO GARCÍA-ALAMILLA GUILLERMO SANDOVAL-ROBLES JOSÉ AARÓN MELO-BANDA LUZ ARCELIA GARCÍA-SERRANO Ingeniería Zirconium oxide Crystallite size Thermal stability Phosphotungstic acid Specific surface area Zirconium hydroxide [Zr(OH)4] was synthesized by the sol-gel method using zirconium n-butoxide and 1-butanol as synthesis precursors. A part of the synthesized material was impregnated with phosphotungstic acid (H3PW12O40) in order to evaluate the effect of this dopant agent on the thermal, textural and structural properties of zirconium oxide (ZrO2). Pure and modified hydroxides were calcined in an air flow at 400, 500 and 600°C for 3 h and afterwards were characterized by thermal analysis, infrared spectroscopy, X-ray diffraction and nitrogen physisorption. Results showed that the interaction between the heteropolyanion and zirconium oxide surface produces a stabilizing effect of the crystalline structure and delays the drastic sintering of the material caused by the thermal treatment, obtaining high specific surface areas and small crystallite size for the modified zirconium oxides. 2014 artículo científico 0012-7353 https://www.redalyc.org/articulo.oa?id=49630072013 en http://www.redalyc.org/revista.oa?id=496 Dyna application/pdf Universidad Nacional de Colombia Dyna (Colombia) Num.183 Vol.81
format Artículo científico
id redalyc_49630072013
institution Redalyc
language en
publishDate 2014
publisher Universidad Nacional de Colombia
spellingShingle EFFECT OF THE ADDITION OF PHOSPHOTUNGSTIC ACID ON THE THERMAL STABILITY OF ZIRCONIUM OXIDE
JUAN MANUEL HERNÁNDEZ-ENRÍQUEZ
Ingeniería
Zirconium oxide
Crystallite size
Thermal stability
Phosphotungstic acid
Specific surface area
EFFECT OF THE ADDITION OF PHOSPHOTUNGSTIC ACID ON THE THERMAL STABILITY OF ZIRCONIUM OXIDE JUAN MANUEL HERNÁNDEZ-ENRÍQUEZ RICARDO GARCÍA-ALAMILLA GUILLERMO SANDOVAL-ROBLES JOSÉ AARÓN MELO-BANDA LUZ ARCELIA GARCÍA-SERRANO Ingeniería Zirconium oxide Crystallite size Thermal stability Phosphotungstic acid Specific surface area Zirconium hydroxide [Zr(OH)4] was synthesized by the sol-gel method using zirconium n-butoxide and 1-butanol as synthesis precursors. A part of the synthesized material was impregnated with phosphotungstic acid (H3PW12O40) in order to evaluate the effect of this dopant agent on the thermal, textural and structural properties of zirconium oxide (ZrO2). Pure and modified hydroxides were calcined in an air flow at 400, 500 and 600°C for 3 h and afterwards were characterized by thermal analysis, infrared spectroscopy, X-ray diffraction and nitrogen physisorption. Results showed that the interaction between the heteropolyanion and zirconium oxide surface produces a stabilizing effect of the crystalline structure and delays the drastic sintering of the material caused by the thermal treatment, obtaining high specific surface areas and small crystallite size for the modified zirconium oxides. 2014 artículo científico 0012-7353 https://www.redalyc.org/articulo.oa?id=49630072013 en http://www.redalyc.org/revista.oa?id=496 Dyna application/pdf Universidad Nacional de Colombia Dyna (Colombia) Num.183 Vol.81
title EFFECT OF THE ADDITION OF PHOSPHOTUNGSTIC ACID ON THE THERMAL STABILITY OF ZIRCONIUM OXIDE
topic Ingeniería
Zirconium oxide
Crystallite size
Thermal stability
Phosphotungstic acid
Specific surface area
url https://www.redalyc.org/articulo.oa?id=49630072013