Simultaneous Passive Water and Electricity Generation in Arid Regions via Fe 3+ /Li + Cross‐Linked Hygroscopic Hydrogels

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Main Authors: Yujie DU, He SHAN, Yongliang ZHENG, Shujing ZHAO, Bin XIE, Yue HAN, Lin YANG, Ruzhu WANG
Format: Artículo Open Access
Published: Wiley 2026
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author Yujie DU
He SHAN
Yongliang ZHENG
Shujing ZHAO
Bin XIE
Yue HAN
Lin YANG
Ruzhu WANG
author_facet Yujie DU
He SHAN
Yongliang ZHENG
Shujing ZHAO
Bin XIE
Yue HAN
Lin YANG
Ruzhu WANG
Yujie DU
He SHAN
Yongliang ZHENG
Shujing ZHAO
Bin XIE
Yue HAN
Lin YANG
Ruzhu WANG
collection Wiley Open Access
contents Simultaneous Passive Water and Electricity Generation in Arid Regions via Fe 3+ /Li + Cross‐Linked Hygroscopic Hydrogels Yujie DU He SHAN Yongliang ZHENG Shujing ZHAO Bin XIE Yue HAN Lin YANG Ruzhu WANG Advanced Materials ABSTRACT Humans are confronting global water scarcity and energy shortages in data centers, and utilizing moisture from the air to address both water and electricity issues is a promising direction. Here, a porous hygroscopic hydrogel is integrated, which is composed of sodium alginate that is co‐loaded with Fe 3+ and Li + . Hydrophilic adsorption sites are constructed via ionic cross‐linking and salt loading, enabling low desorption enthalpy (<40 kJ mol − 1 ) for efficient water desorption. The water uptake of the dual‐ionic hydrogel is over 5.1 g g −1 at 90% RH, and this value is 1.1 g g −1 at 30% RH. By designing a water harvesting device with rotating adsorption/desorption zones, with a daily production of 11.8 L kg hydrogel −1 at 70% RH. The hydrogel not only provides abundant sites for moisture adsorption and storage but also offers channels for ion transport to enhance electricity generation. By constructing an asymmetric humidity structure, the dissociated cations in the hydrogel will diffusion to the substrate by concentration gradient and the electricity is evocated, producing a highly short‐circuit current (250 µA) and open‐circuit voltage (7.6 V), illuminating the multi‐LED lights. 10.1002/adma.73439 http://onlinelibrary.wiley.com/termsAndConditions#vor
doi_str_mv 10.1002/adma.73439
format Artículo Open Access
id wiley_oa_10_1002_adma_73439
institution Wiley Open Access
license_str_mv http://onlinelibrary.wiley.com/termsAndConditions#vor
publishDate 2026
publisher Wiley
record_format wiley_oa
spellingShingle Simultaneous Passive Water and Electricity Generation in Arid Regions via Fe 3+ /Li + Cross‐Linked Hygroscopic Hydrogels
Yujie DU
He SHAN
Yongliang ZHENG
Shujing ZHAO
Bin XIE
Yue HAN
Lin YANG
Ruzhu WANG
Advanced Materials
Simultaneous Passive Water and Electricity Generation in Arid Regions via Fe 3+ /Li + Cross‐Linked Hygroscopic Hydrogels Yujie DU He SHAN Yongliang ZHENG Shujing ZHAO Bin XIE Yue HAN Lin YANG Ruzhu WANG Advanced Materials ABSTRACT Humans are confronting global water scarcity and energy shortages in data centers, and utilizing moisture from the air to address both water and electricity issues is a promising direction. Here, a porous hygroscopic hydrogel is integrated, which is composed of sodium alginate that is co‐loaded with Fe 3+ and Li + . Hydrophilic adsorption sites are constructed via ionic cross‐linking and salt loading, enabling low desorption enthalpy (<40 kJ mol − 1 ) for efficient water desorption. The water uptake of the dual‐ionic hydrogel is over 5.1 g g −1 at 90% RH, and this value is 1.1 g g −1 at 30% RH. By designing a water harvesting device with rotating adsorption/desorption zones, with a daily production of 11.8 L kg hydrogel −1 at 70% RH. The hydrogel not only provides abundant sites for moisture adsorption and storage but also offers channels for ion transport to enhance electricity generation. By constructing an asymmetric humidity structure, the dissociated cations in the hydrogel will diffusion to the substrate by concentration gradient and the electricity is evocated, producing a highly short‐circuit current (250 µA) and open‐circuit voltage (7.6 V), illuminating the multi‐LED lights. 10.1002/adma.73439 http://onlinelibrary.wiley.com/termsAndConditions#vor
title Simultaneous Passive Water and Electricity Generation in Arid Regions via Fe 3+ /Li + Cross‐Linked Hygroscopic Hydrogels
topic Advanced Materials
url https://advanced.onlinelibrary.wiley.com/doi/10.1002/adma.73439