High‐Sensitivity Perovskite γ‐Ray Detectors Enhanced by Device Engineering Toward Energy Spectroscopy Imaging

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Autori principali: Ken Qin, Jia‐He Zhang, Ruo‐Long Zhou, Xue Sun, He‐Xuan Wang, Jia‐Li Peng, Min‐Shu Zhang, Guan‐Hua Dun, Dan Xie, He Tian, Yi Yang, Tian‐Ling Ren
Natura: Artículo Open Access
Pubblicazione: Wiley 2025
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author Ken Qin
Jia‐He Zhang
Ruo‐Long Zhou
Xue Sun
He‐Xuan Wang
Jia‐Li Peng
Min‐Shu Zhang
Guan‐Hua Dun
Dan Xie
He Tian
Yi Yang
Tian‐Ling Ren
author_facet Ken Qin
Jia‐He Zhang
Ruo‐Long Zhou
Xue Sun
He‐Xuan Wang
Jia‐Li Peng
Min‐Shu Zhang
Guan‐Hua Dun
Dan Xie
He Tian
Yi Yang
Tian‐Ling Ren
Ken Qin
Jia‐He Zhang
Ruo‐Long Zhou
Xue Sun
He‐Xuan Wang
Jia‐Li Peng
Min‐Shu Zhang
Guan‐Hua Dun
Dan Xie
He Tian
Yi Yang
Tian‐Ling Ren
collection Wiley Open Access
contents High‐Sensitivity Perovskite γ‐Ray Detectors Enhanced by Device Engineering Toward Energy Spectroscopy Imaging Ken Qin Jia‐He Zhang Ruo‐Long Zhou Xue Sun He‐Xuan Wang Jia‐Li Peng Min‐Shu Zhang Guan‐Hua Dun Dan Xie He Tian Yi Yang Tian‐Ling Ren Advanced Science Abstract Perovskite‐based detectors for γ‐rays have emerged relatively recently and have attracted limited attention. Although increasing efforts are being directed towards their development, the absence of an adaptive processor, systematic theoretical framework, and various applications limit its further development. In this paper, drawing inspiration from the commercial detectors, electrode configuration is improved to reshape the bias electric field, guide the effective signal carrier, and mitigate the noise from the side section. Through theoretical analysis, simulations, and experimental comparisons, the clear improvement of energy resolution from 7% to ≈5% is demonstrated, and the highest resolution of 1.9% is observed. Furthermore, to fill up the research framework of radiation, the definition of X‐ray sensitivity is extended to quantitatively describe the γ‐ray response, and assess the performance of γ‐ray detectors, reaching a sensitivity ≈10 5 µC Gy air −1 cm −2 . Based on these, a spectral‐enhanced imaging strategy is proposed to broaden the application of γ‐Ray detectors, where the spectral dimension of images is utilized to improve contrast and enhance imaging quality. 10.1002/advs.202503597 http://creativecommons.org/licenses/by/4.0/
doi_str_mv 10.1002/advs.202503597
format Artículo Open Access
id wiley_oa_10_1002_advs_202503597
institution Wiley Open Access
license_str_mv http://creativecommons.org/licenses/by/4.0/
publishDate 2025
publisher Wiley
record_format wiley_oa
spellingShingle High‐Sensitivity Perovskite γ‐Ray Detectors Enhanced by Device Engineering Toward Energy Spectroscopy Imaging
Ken Qin
Jia‐He Zhang
Ruo‐Long Zhou
Xue Sun
He‐Xuan Wang
Jia‐Li Peng
Min‐Shu Zhang
Guan‐Hua Dun
Dan Xie
He Tian
Yi Yang
Tian‐Ling Ren
Advanced Science
High‐Sensitivity Perovskite γ‐Ray Detectors Enhanced by Device Engineering Toward Energy Spectroscopy Imaging Ken Qin Jia‐He Zhang Ruo‐Long Zhou Xue Sun He‐Xuan Wang Jia‐Li Peng Min‐Shu Zhang Guan‐Hua Dun Dan Xie He Tian Yi Yang Tian‐Ling Ren Advanced Science Abstract Perovskite‐based detectors for γ‐rays have emerged relatively recently and have attracted limited attention. Although increasing efforts are being directed towards their development, the absence of an adaptive processor, systematic theoretical framework, and various applications limit its further development. In this paper, drawing inspiration from the commercial detectors, electrode configuration is improved to reshape the bias electric field, guide the effective signal carrier, and mitigate the noise from the side section. Through theoretical analysis, simulations, and experimental comparisons, the clear improvement of energy resolution from 7% to ≈5% is demonstrated, and the highest resolution of 1.9% is observed. Furthermore, to fill up the research framework of radiation, the definition of X‐ray sensitivity is extended to quantitatively describe the γ‐ray response, and assess the performance of γ‐ray detectors, reaching a sensitivity ≈10 5 µC Gy air −1 cm −2 . Based on these, a spectral‐enhanced imaging strategy is proposed to broaden the application of γ‐Ray detectors, where the spectral dimension of images is utilized to improve contrast and enhance imaging quality. 10.1002/advs.202503597 http://creativecommons.org/licenses/by/4.0/
title High‐Sensitivity Perovskite γ‐Ray Detectors Enhanced by Device Engineering Toward Energy Spectroscopy Imaging
topic Advanced Science
url https://advanced.onlinelibrary.wiley.com/doi/10.1002/advs.202503597