Sustainable Carbon‐Based Catalyst Materials Derived From Lignocellulosic Biomass for Energy Storage and Conversion: Atomic Modulation and Properties Improvement

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Main Authors: Wei Li, Ying Xu, Guanhua Wang, Ting Xu, Kui Wang, Shangru Zhai, Chuanling Si
Format: Artículo Open Access
Published: Wiley 2025
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author Wei Li
Ying Xu
Guanhua Wang
Ting Xu
Kui Wang
Shangru Zhai
Chuanling Si
author_facet Wei Li
Ying Xu
Guanhua Wang
Ting Xu
Kui Wang
Shangru Zhai
Chuanling Si
Wei Li
Ying Xu
Guanhua Wang
Ting Xu
Kui Wang
Shangru Zhai
Chuanling Si
collection Wiley Open Access
contents Sustainable Carbon‐Based Catalyst Materials Derived From Lignocellulosic Biomass for Energy Storage and Conversion: Atomic Modulation and Properties Improvement Wei Li Ying Xu Guanhua Wang Ting Xu Kui Wang Shangru Zhai Chuanling Si Carbon Energy ABSTRACTCarbon electrocatalyst materials based on lignocellulosic biomass with multi‐components, various dimensions, high carbon content, and hierarchical morphology structures have gained great popularity in electrocatalytic applications recently. Due to the catalytic deficiency of neutral carbon atoms, the usage of single lignocellulosic‐based carbon materials in electrocatalysis involving energy storage and conversion presents unsatisfactory applicability. However, atomic‐level modulation of lignocellulose‐based carbon materials can optimize the electronic structures, charge separation, transfer processes, and so forth, which results in substantially enhanced electrocatalytic performance of carbon‐based catalysts. This paper reviews the recent advances in the rational design of lignocellulosic‐based carbon materials as electrocatalysts from an atomic‐level perspective, such as self/external heteroatom doping and metal modification. Then, through systematic discussion of the design principles and reaction mechanisms of the catalysts, the applications of the prepared lignocellulosic‐based catalysts in rechargeable batteries and electrocatalysis are reviewed. Finally, the challenges in improving the catalytic performance of lignocellulosic‐based carbon materials as electrocatalysts and the prospects in diverse applications are reviewed. This review contributes to the synthesis strategy of lignocellulose‐based carbon electrocatalysts via atomic‐level modulation, which in turn promotes the lignocellulose valorization for energy storage and conversion. 10.1002/cey2.708 http://creativecommons.org/licenses/by/4.0/
doi_str_mv 10.1002/cey2.708
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institution Wiley Open Access
license_str_mv http://creativecommons.org/licenses/by/4.0/
publishDate 2025
publisher Wiley
record_format wiley_oa
spellingShingle Sustainable Carbon‐Based Catalyst Materials Derived From Lignocellulosic Biomass for Energy Storage and Conversion: Atomic Modulation and Properties Improvement
Wei Li
Ying Xu
Guanhua Wang
Ting Xu
Kui Wang
Shangru Zhai
Chuanling Si
Carbon Energy
Sustainable Carbon‐Based Catalyst Materials Derived From Lignocellulosic Biomass for Energy Storage and Conversion: Atomic Modulation and Properties Improvement Wei Li Ying Xu Guanhua Wang Ting Xu Kui Wang Shangru Zhai Chuanling Si Carbon Energy ABSTRACTCarbon electrocatalyst materials based on lignocellulosic biomass with multi‐components, various dimensions, high carbon content, and hierarchical morphology structures have gained great popularity in electrocatalytic applications recently. Due to the catalytic deficiency of neutral carbon atoms, the usage of single lignocellulosic‐based carbon materials in electrocatalysis involving energy storage and conversion presents unsatisfactory applicability. However, atomic‐level modulation of lignocellulose‐based carbon materials can optimize the electronic structures, charge separation, transfer processes, and so forth, which results in substantially enhanced electrocatalytic performance of carbon‐based catalysts. This paper reviews the recent advances in the rational design of lignocellulosic‐based carbon materials as electrocatalysts from an atomic‐level perspective, such as self/external heteroatom doping and metal modification. Then, through systematic discussion of the design principles and reaction mechanisms of the catalysts, the applications of the prepared lignocellulosic‐based catalysts in rechargeable batteries and electrocatalysis are reviewed. Finally, the challenges in improving the catalytic performance of lignocellulosic‐based carbon materials as electrocatalysts and the prospects in diverse applications are reviewed. This review contributes to the synthesis strategy of lignocellulose‐based carbon electrocatalysts via atomic‐level modulation, which in turn promotes the lignocellulose valorization for energy storage and conversion. 10.1002/cey2.708 http://creativecommons.org/licenses/by/4.0/
title Sustainable Carbon‐Based Catalyst Materials Derived From Lignocellulosic Biomass for Energy Storage and Conversion: Atomic Modulation and Properties Improvement
topic Carbon Energy
url https://onlinelibrary.wiley.com/doi/10.1002/cey2.708