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| Main Authors: | , , , , , , , |
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| Format: | Artículo Open Access |
| Published: |
Wiley
2024
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| Subjects: | |
| Online Access: | https://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/cssc.202401708 |
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Table of Contents:
- Novel Graphitic Oxynitrides as Photocatalysts for Sustainable H2 Production and CO2 Valorization. The Importance of Self‐Assembly for Catalytic Activity Nieves Lavado Rosario Pardo‐Botello José María Sánchez‐Rodas R. Fernando Martínez Vicente Montes Francisco Javier López‐Tenllado Pedro Cintas Reyes Babiano ChemSusChem AbstractThe field of carbocatalysis, often portrayed by paradigmatic graphitic carbonaceous structures, has become a booming topic tailored for multiple applications. To this end, a new metal‐free carbocatalyst has been constructed from simple prebiotic monomers such as cyanamide and glyoxal. The resulting material shows an excellent performance as photocatalyst for H2 production and CO2 valorization, thus unveiling its real value to tackle sustainable goals. The unique oxygen‐rich carbonaceous structure has been characterized in detail, which is consistent with a graphitic layered network. The described performance in two major societal concerns along with a facile preparation from C1/C2 platforms, makes this type of overlooked oxynitride carbocatalysts promising for real‐life environmental endeavors. 10.1002/cssc.202401708 http://creativecommons.org/licenses/by-nc-nd/4.0/