Ultrasonication‐Assisted Single Hybrid Solar‐Light Active Nanocomposite Photocatalyst/Biocatalyst Enabling Artificial Photosynthesis for Solar CO 2 ‐to‐Formic Acid Conversion
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| Format: | Artículo Open Access |
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Wiley
2026
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| author | Rahul Maddheshiya Rajesh K. Yadav Rajesh K. Verma Chinna Bathula Kanchan Sharma Geeta Srivastava Anupma Yadav Shaifali Mishra Rehana Shahin Arun Kumar Dubey Jin OoK Baeg |
| author_facet | Rahul Maddheshiya Rajesh K. Yadav Rajesh K. Verma Chinna Bathula Kanchan Sharma Geeta Srivastava Anupma Yadav Shaifali Mishra Rehana Shahin Arun Kumar Dubey Jin OoK Baeg Rahul Maddheshiya Rajesh K. Yadav Rajesh K. Verma Chinna Bathula Kanchan Sharma Geeta Srivastava Anupma Yadav Shaifali Mishra Rehana Shahin Arun Kumar Dubey Jin OoK Baeg |
| collection | Wiley Open Access |
| contents | Ultrasonication‐Assisted Single Hybrid Solar‐Light Active Nanocomposite Photocatalyst/Biocatalyst Enabling Artificial Photosynthesis for Solar CO 2 ‐to‐Formic Acid Conversion Rahul Maddheshiya Rajesh K. Yadav Rajesh K. Verma Chinna Bathula Kanchan Sharma Geeta Srivastava Anupma Yadav Shaifali Mishra Rehana Shahin Arun Kumar Dubey Jin OoK Baeg ChemistrySelect ABSTRACT Using CO 2 with an affordable technique is an exciting challenge for scientists. So, in this study, we introduce the creation of a budget‐friendly, ultrasonication‐assisted single hybrid solar‐light active SeGCN@Fe 3 O 4 nanocomposite photocatalyst enabling an artificial photosynthetic system for solar CO 2 ‐to‐formic acid conversion. This present research highlights the innovation of a facile ultrasonication‐driven synthesis incorporating magnetic Fe 3 O 4 and Se doping into a single hybrid system, enhancing charge separation, absorption of light, and providing easy magnetic recovery. This ultrasonication‐assisted single hybrid solar‐light active nanocomposite catalyst, combined with a biocatalyst system, works in a very selective way, achieving a high NADH regeneration of 94.17 %, which is then used to produce pure formic acid from CO 2 (225.18 µM, Quantum efficiency; η = 2.817%). Moreover, the integration of photocatalysis with a biocatalytic process provides a simple and highly effective artificial photosynthetic platform, without the need for a complex multicomponent system. This combined approach, our work, ecstatically emphasizes the growth and use of a SeGCN‐based photocatalyst for directly turning carbon dioxide into solar fuels. 10.1002/slct.73439 http://onlinelibrary.wiley.com/termsAndConditions#vor |
| doi_str_mv | 10.1002/slct.73439 |
| format | Artículo Open Access |
| id | wiley_oa_10_1002_slct_73439 |
| institution | Wiley Open Access |
| license_str_mv | http://onlinelibrary.wiley.com/termsAndConditions#vor |
| publishDate | 2026 |
| publisher | Wiley |
| record_format | wiley_oa |
| spellingShingle | Ultrasonication‐Assisted Single Hybrid Solar‐Light Active Nanocomposite Photocatalyst/Biocatalyst Enabling Artificial Photosynthesis for Solar CO 2 ‐to‐Formic Acid Conversion Rahul Maddheshiya Rajesh K. Yadav Rajesh K. Verma Chinna Bathula Kanchan Sharma Geeta Srivastava Anupma Yadav Shaifali Mishra Rehana Shahin Arun Kumar Dubey Jin OoK Baeg ChemistrySelect Ultrasonication‐Assisted Single Hybrid Solar‐Light Active Nanocomposite Photocatalyst/Biocatalyst Enabling Artificial Photosynthesis for Solar CO 2 ‐to‐Formic Acid Conversion Rahul Maddheshiya Rajesh K. Yadav Rajesh K. Verma Chinna Bathula Kanchan Sharma Geeta Srivastava Anupma Yadav Shaifali Mishra Rehana Shahin Arun Kumar Dubey Jin OoK Baeg ChemistrySelect ABSTRACT Using CO 2 with an affordable technique is an exciting challenge for scientists. So, in this study, we introduce the creation of a budget‐friendly, ultrasonication‐assisted single hybrid solar‐light active SeGCN@Fe 3 O 4 nanocomposite photocatalyst enabling an artificial photosynthetic system for solar CO 2 ‐to‐formic acid conversion. This present research highlights the innovation of a facile ultrasonication‐driven synthesis incorporating magnetic Fe 3 O 4 and Se doping into a single hybrid system, enhancing charge separation, absorption of light, and providing easy magnetic recovery. This ultrasonication‐assisted single hybrid solar‐light active nanocomposite catalyst, combined with a biocatalyst system, works in a very selective way, achieving a high NADH regeneration of 94.17 %, which is then used to produce pure formic acid from CO 2 (225.18 µM, Quantum efficiency; η = 2.817%). Moreover, the integration of photocatalysis with a biocatalytic process provides a simple and highly effective artificial photosynthetic platform, without the need for a complex multicomponent system. This combined approach, our work, ecstatically emphasizes the growth and use of a SeGCN‐based photocatalyst for directly turning carbon dioxide into solar fuels. 10.1002/slct.73439 http://onlinelibrary.wiley.com/termsAndConditions#vor |
| title | Ultrasonication‐Assisted Single Hybrid Solar‐Light Active Nanocomposite Photocatalyst/Biocatalyst Enabling Artificial Photosynthesis for Solar CO 2 ‐to‐Formic Acid Conversion |
| topic | ChemistrySelect |
| url | https://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/slct.73439 |