Long‐Range Trion Guides in Strain‐Engineered Atomically Thin Semiconductor

Fuente: Wiley Open Access
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Auteurs principaux: Wenqi Qian, Xueying Wang, Haiyi Liu, Guangyi Tao, Fangxun Liu, Sihan Lin, Tengteng Gao, Lie Lin, Pengfei Qi, Zheyu Fang, Weiwei Liu
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Publié: Wiley 2025
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author Wenqi Qian
Xueying Wang
Haiyi Liu
Guangyi Tao
Fangxun Liu
Sihan Lin
Tengteng Gao
Lie Lin
Pengfei Qi
Zheyu Fang
Weiwei Liu
author_facet Wenqi Qian
Xueying Wang
Haiyi Liu
Guangyi Tao
Fangxun Liu
Sihan Lin
Tengteng Gao
Lie Lin
Pengfei Qi
Zheyu Fang
Weiwei Liu
Wenqi Qian
Xueying Wang
Haiyi Liu
Guangyi Tao
Fangxun Liu
Sihan Lin
Tengteng Gao
Lie Lin
Pengfei Qi
Zheyu Fang
Weiwei Liu
collection Wiley Open Access
contents Long‐Range Trion Guides in Strain‐Engineered Atomically Thin Semiconductor Wenqi Qian Xueying Wang Haiyi Liu Guangyi Tao Fangxun Liu Sihan Lin Tengteng Gao Lie Lin Pengfei Qi Zheyu Fang Weiwei Liu Small Structures Exciton‐based devices offer a compelling route to address the trade‐off between integration density and response speed faced by electronic and photonic systems. In atomically thin transition metal dichalcogenide, excitons exhibit remarkable binding strength together with adjustable valley characteristics, which makes it possible to explore excitonic behaviors and realize device functionalities at room temperature. However, realizing directional exciton motion within atomically thin semiconductors remains a challenge due to their intrinsic isotropic diffusion nature, which limit the transport efficiency of excitons in specific directions. Here, the capillary force‐assisted technique is proposed to fabricate long‐range trion guides in atomically thin semiconductors, enabling the direct visualization of oriented exciton transport. Exciton funneling and exciton‐to‐trion conversion in heterostructure of WSe 2 monolayer transferred on SiC nanowire to create strain gradients are demonstrated by micro photoluminescence (PL) mappings and first‐principle calculations. An unusual remote emission effect—where PL appears nearly 10 μm distant from the excitation spot—is detected, and this behavior is ascribed to the strain‐engineered potential profile that confines trions within the 1D pathway and directs their transport away from the excitation region. These results offer new insights into directional trion guiding within 2D semiconductors. 10.1002/sstr.202500406 http://creativecommons.org/licenses/by/4.0/
doi_str_mv 10.1002/sstr.202500406
format Artículo Open Access
id wiley_oa_10_1002_sstr_202500406
institution Wiley Open Access
license_str_mv http://creativecommons.org/licenses/by/4.0/
publishDate 2025
publisher Wiley
record_format wiley_oa
spellingShingle Long‐Range Trion Guides in Strain‐Engineered Atomically Thin Semiconductor
Wenqi Qian
Xueying Wang
Haiyi Liu
Guangyi Tao
Fangxun Liu
Sihan Lin
Tengteng Gao
Lie Lin
Pengfei Qi
Zheyu Fang
Weiwei Liu
Small Structures
Long‐Range Trion Guides in Strain‐Engineered Atomically Thin Semiconductor Wenqi Qian Xueying Wang Haiyi Liu Guangyi Tao Fangxun Liu Sihan Lin Tengteng Gao Lie Lin Pengfei Qi Zheyu Fang Weiwei Liu Small Structures Exciton‐based devices offer a compelling route to address the trade‐off between integration density and response speed faced by electronic and photonic systems. In atomically thin transition metal dichalcogenide, excitons exhibit remarkable binding strength together with adjustable valley characteristics, which makes it possible to explore excitonic behaviors and realize device functionalities at room temperature. However, realizing directional exciton motion within atomically thin semiconductors remains a challenge due to their intrinsic isotropic diffusion nature, which limit the transport efficiency of excitons in specific directions. Here, the capillary force‐assisted technique is proposed to fabricate long‐range trion guides in atomically thin semiconductors, enabling the direct visualization of oriented exciton transport. Exciton funneling and exciton‐to‐trion conversion in heterostructure of WSe 2 monolayer transferred on SiC nanowire to create strain gradients are demonstrated by micro photoluminescence (PL) mappings and first‐principle calculations. An unusual remote emission effect—where PL appears nearly 10 μm distant from the excitation spot—is detected, and this behavior is ascribed to the strain‐engineered potential profile that confines trions within the 1D pathway and directs their transport away from the excitation region. These results offer new insights into directional trion guiding within 2D semiconductors. 10.1002/sstr.202500406 http://creativecommons.org/licenses/by/4.0/
title Long‐Range Trion Guides in Strain‐Engineered Atomically Thin Semiconductor
topic Small Structures
url https://onlinelibrary.wiley.com/doi/10.1002/sstr.202500406