FATTY ACID-BASED DIISOCYANATE SYNTHESIS FOR THE PRODUCTION OF GREEN POLYURETHANES

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Main Authors: Andrade, Ângela G. L. L., Pezzin, Sérgio
Format: Recurso digital
Language:English
Published: Zenodo 2023
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author Andrade, Ângela G. L. L.
Pezzin, Sérgio
author_facet Andrade, Ângela G. L. L.
Pezzin, Sérgio
contents <p>Aiming to the development of new synthetic routes for polyurethanes (PU) from raw materials exclusively from renewable sources, a 'green' synthesis of 1,8-diisocyanatooctane (DIO) was carried out from fatty acid derivatives by a method without the use of phosgene. The three-step synthetic route started from dimethyl sebacate, with the preparation of decanedihydrazide and decanedioyl diazide as intermediates, under nitrogen atmosphere. FTIR and ¹H NMR analyses confirmed the structure of the diisocyanate, which is a promising 'green' alternative to be used in the production of more sustainable polyurethanes by reaction with suitable polyols from biomass.</p>
format Recurso digital
id zenodo_https___doi_org_10_5281_zenodo_15701385
institution Zenodo
language eng
publishDate 2023
publisher Zenodo
record_format zenodo
spellingShingle FATTY ACID-BASED DIISOCYANATE SYNTHESIS FOR THE PRODUCTION OF GREEN POLYURETHANES
Andrade, Ângela G. L. L.
Pezzin, Sérgio
Isocyanates/chemical synthesis
Fatty Acids
renewable sources
green synthesis
<p>Aiming to the development of new synthetic routes for polyurethanes (PU) from raw materials exclusively from renewable sources, a 'green' synthesis of 1,8-diisocyanatooctane (DIO) was carried out from fatty acid derivatives by a method without the use of phosgene. The three-step synthetic route started from dimethyl sebacate, with the preparation of decanedihydrazide and decanedioyl diazide as intermediates, under nitrogen atmosphere. FTIR and ¹H NMR analyses confirmed the structure of the diisocyanate, which is a promising 'green' alternative to be used in the production of more sustainable polyurethanes by reaction with suitable polyols from biomass.</p>
title FATTY ACID-BASED DIISOCYANATE SYNTHESIS FOR THE PRODUCTION OF GREEN POLYURETHANES
topic Isocyanates/chemical synthesis
Fatty Acids
renewable sources
green synthesis
url https://doi.org/10.5281/zenodo.15701385