Parametric Phase-Locking of Hydrogen-Bond Networks: High-Frequency Floquet Dressing of Liquid Water Topology
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| Format: | Recurso digital |
| Language: | English |
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Zenodo
2026
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| _version_ | 1866901095610056704 |
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| author | Claudia Attaianese |
| author_facet | Claudia Attaianese |
| contents | <p>This work presents a theoretical framework for dynamically modifying the structural dynamics of liquid water using high-frequency parametric driving.</p> <p>Modeling water as a dense network of interacting dipolar rotors, we analyze the effect of a fast, coherent electromagnetic field in the multi-terahertz regime using Floquet averaging techniques.</p> <p>We show that high-frequency driving induces a renormalization of dipole-dipole interactions via a Bessel-function dependence, effectively modifying the orientational energy landscape.</p> <p>This mechanism can significantly reduce rotational diffusion and extend hydrogen-bond lifetimes, leading to a transition toward a long-lived prethermal regime with enhanced structural correlations.</p> <p>The model predicts a crossover from rapidly decorrelating liquid dynamics to a dynamically stabilized state with increased tetrahedral ordering under sufficiently strong driving.</p> <p>This work provides a physically motivated framework for controlling the dynamics and topology of dipolar liquids through non-equilibrium parametric forcing.</p> |
| format | Recurso digital |
| id | zenodo_https___doi_org_10_5281_zenodo_19204400 |
| institution | Zenodo |
| language | eng |
| publishDate | 2026 |
| publisher | Zenodo |
| record_format | zenodo |
| spellingShingle | Parametric Phase-Locking of Hydrogen-Bond Networks: High-Frequency Floquet Dressing of Liquid Water Topology Claudia Attaianese liquid water hydrogen bonding dipolar interactions Floquet theory nonlinear dynamics statistical physics parametric stabilization orientational dynamics complex systems non-equilibrium systems <p>This work presents a theoretical framework for dynamically modifying the structural dynamics of liquid water using high-frequency parametric driving.</p> <p>Modeling water as a dense network of interacting dipolar rotors, we analyze the effect of a fast, coherent electromagnetic field in the multi-terahertz regime using Floquet averaging techniques.</p> <p>We show that high-frequency driving induces a renormalization of dipole-dipole interactions via a Bessel-function dependence, effectively modifying the orientational energy landscape.</p> <p>This mechanism can significantly reduce rotational diffusion and extend hydrogen-bond lifetimes, leading to a transition toward a long-lived prethermal regime with enhanced structural correlations.</p> <p>The model predicts a crossover from rapidly decorrelating liquid dynamics to a dynamically stabilized state with increased tetrahedral ordering under sufficiently strong driving.</p> <p>This work provides a physically motivated framework for controlling the dynamics and topology of dipolar liquids through non-equilibrium parametric forcing.</p> |
| title | Parametric Phase-Locking of Hydrogen-Bond Networks: High-Frequency Floquet Dressing of Liquid Water Topology |
| topic | liquid water hydrogen bonding dipolar interactions Floquet theory nonlinear dynamics statistical physics parametric stabilization orientational dynamics complex systems non-equilibrium systems |
| url | https://doi.org/10.5281/zenodo.19204400 |