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Main Authors: Wei, Yicheng, Xu, Han, Zhang, Xingqiang, Wang, Wei, Cheng, Zhe
Format: Preprint
Published: 2026
Subjects:
Online Access:https://arxiv.org/abs/2603.03737
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author Wei, Yicheng
Xu, Han
Zhang, Xingqiang
Wang, Wei
Cheng, Zhe
author_facet Wei, Yicheng
Xu, Han
Zhang, Xingqiang
Wang, Wei
Cheng, Zhe
contents Parylene C thin films have significant applications in advanced packaging of microelectronics. Their thermal properties are critical for thermal management of electronic devices. However, a unified understanding of the tunable structure and the corresponding thermal conductivity is still missing. This study investigated parylene C thin films of varying thickness and post-annealing temperatures grown via thermal chemical vapor deposition. The ultralow thermal conductivity of as-deposited parylene C measured by time domain thermoreflectance (TDTR) is 0.10 W/m-K. The thermal conductivity can be tuned by post-annealing. Significant increase in thermal conductivity is observed in the annealed samples (0.18 W/m-K) which induces melting and recrystallization. The results of XRD and polarized Raman spectroscopy show that the enhanced thermal conductivity is due to improved crystalline quality and the change in chain orientations. The measured thermal conductivities of the as-deposited and annealed films are much lower than the values predicted by the Cahill minimum thermal conductivity model, which can be explained by the diffuson-mediated minimum thermal conductivity model. Parylene C is found to possess the lowest thermal conductivity among dense low-k materials. Our work provides guidance for the structural design of ultra-low thermal conductivity polymers and corresponding thermal design of electronics.
format Preprint
id arxiv_https___arxiv_org_abs_2603_03737
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Ultralow and Tunable Thermal Conductivity of Parylene C for Thermal Insulation in Advanced Packaging
Wei, Yicheng
Xu, Han
Zhang, Xingqiang
Wang, Wei
Cheng, Zhe
Materials Science
Applied Physics
Parylene C thin films have significant applications in advanced packaging of microelectronics. Their thermal properties are critical for thermal management of electronic devices. However, a unified understanding of the tunable structure and the corresponding thermal conductivity is still missing. This study investigated parylene C thin films of varying thickness and post-annealing temperatures grown via thermal chemical vapor deposition. The ultralow thermal conductivity of as-deposited parylene C measured by time domain thermoreflectance (TDTR) is 0.10 W/m-K. The thermal conductivity can be tuned by post-annealing. Significant increase in thermal conductivity is observed in the annealed samples (0.18 W/m-K) which induces melting and recrystallization. The results of XRD and polarized Raman spectroscopy show that the enhanced thermal conductivity is due to improved crystalline quality and the change in chain orientations. The measured thermal conductivities of the as-deposited and annealed films are much lower than the values predicted by the Cahill minimum thermal conductivity model, which can be explained by the diffuson-mediated minimum thermal conductivity model. Parylene C is found to possess the lowest thermal conductivity among dense low-k materials. Our work provides guidance for the structural design of ultra-low thermal conductivity polymers and corresponding thermal design of electronics.
title Ultralow and Tunable Thermal Conductivity of Parylene C for Thermal Insulation in Advanced Packaging
topic Materials Science
Applied Physics
url https://arxiv.org/abs/2603.03737